ISSN 1063-7826, Semiconductors, 2014, Vol. 48, No. 9, pp. 1242–1247. © Pleiades Publishing, Ltd., 2014.
Original Russian Text © A.P. Dostanko, O.A. Ageev, D.A. Golosov, S.M. Zavadski, E.G. Zamburg, D.E. Vakulov, Z.E. Vakulov, 2014, published in Fizika i Tekhnika Poluprovodnikov,
2014, Vol. 48, No. 9, pp. 1274–1279.
1242
1. INTRODUCTION
In recent years, renewed interest in thin-film zinc
oxide (ZnO) layers has been noted. The increased
interest in this field is caused by the unique combina-
tion of optical and electrical properties of zinc oxide.
Zinc-oxide films that possess a high degree of chemi-
cal inertness and resistance to atmospheric effects are
used as conductive coatings, transparent in the infra-
red (IR) and visible spectral regions, for electrical con-
tacts and buffer layers of thin-film solar cells and
information display units [1, 2]. The doping of ZnO
films makes it possible to attain a resistivity up to 2 ×
10
–4
Ω cm [3, 4]. Zinc-oxide films possess good piezo-
electric and electroluminescence characteristics and
can be used as functional layers in devices, whose
operation is based on surface acoustic waves [5, 6],
sources and detectors of ultraviolet (UV) and IR radi-
ation, optical shutters, and nonlinear optical elements
[7–9]. The ability of heated ZnO films to adsorb cer-
tain gases and, in this case, to change conductivity
makes possible the use of these films as active elements
of gas sensors [10].
The widespread industrial use of devices based on
ZnO layers is limited by the complexity of the produc-
tion of ZnO films with specified functional character-
istics. Zinc oxide belongs to the group of direct-gap
semiconductors, and the properties of the deposited
films depend to a large extent on the concentration of
free charge carriers controlled by oxygen vacancies
[2].
The currently most widely applied method of the
formation of thin-film ZnO layers is reactive magne-
tron sputtering [11, 12]. This technique provides a
means for varying the conditions of film deposition
within wide limits and, thus, for controlling the elec-
trical and structural properties of the deposited coat-
ing. Among the disadvantages of this technique, the
complexity of the production of stoichiometric layers
without heating the substrates must be mentioned.
The magnetron sputtering procedures developed thus
far provide the production of ZnO layers at tempera-
tures higher than 200°C, which restricts the field of
possible applications of the layers [13]. For example,
in the case of deposition onto polymeric substrates,
the temperature during deposition of the films must be
no higher than 80–120°C (the typical temperatures
are 70–80°C). In addition, it is found that, in the case
of the magnetron deposition of ZnO films, the distri-
bution of the optical and electrical characteristics of
the resulting ZnO layers is nonuniform because of
bombardment of the growing film by high-energy neg-
ative oxygen ions and atoms [14].
At the same time, inadequate attention is given to
the use of the ion-beam sputtering of oxide targets.
This technique provides deposition rates comparable
to those in the above-mentioned technique [15] and
the formation of stoichiometric layers without heating
of the substrate. In addition, the technique allows
comparatively easy scaling [16].
Thus, the purpose of this study is to explore the
electrical and optical characteristics of ZnO films
deposited by the ion-beam sputtering of a ZnO oxide
target without heating of the substrate.
Electrical and Optical Properties of Zinc-Oxide Films Deposited
by the Ion-Beam Sputtering of an Oxide Target
A. P. Dostanko
a
, O. A. Ageev
b
, D. A. Golosov
a
^, S. M. Zavadski
a
,
E. G. Zamburg
b
, D. E. Vakulov
b
, and Z. E. Vakulov
b
a
Belarusian State University of Informatics and Radioelectronics, Minsk, 220013 Belarus
^e-mail: dmgolosov@gmail.com
b
Southern Federal University, Taganrog, 347928 Russia
Submitted November 25, 2013; accepted for publication December 3, 2013
Abstract—The influence of the parameters of the deposition process on the stoichiometric composition and
electrical and optical properties of ZnO films deposited by the ion-beam sputtering of a ZnO target is studied.
It is established that, upon sputtering of a ZnO target with stoichiometric composition, there is a deficit of
oxygen in the films deposited. Even for the case of target sputtering in a pure O
2
atmosphere, the stoichiom-
etry index of the films is no higher than 0.98. A decrease in the oxygen content in the films is accompanied
by a sharp decrease in the resistivity to 35–40 Ω m, narrowing of the optical band gap, and a shift of the optical
transmittance edge from 389 to 404 nm. All of the variations in the optical and electrical properties of the ZnO
films can be attributed to variations in the concentration and mobility of free charge carriers in the films.
DOI: 10.1134/S1063782614090073
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