© 2014 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim
Phys. Status Solidi RRL, 1–4 (2014) / DOI 10.1002/pssr.201409295
The effect of annealing ambient
on carrier recombination
in boron implanted silicon
Thomas Ratcliff
*, 1
, Kean Chern Fong
1
, Avi Shalav
2
, Robert Elliman
2
, and Andrew Blakers
1
1
Centre for Sustainable Energy Systems, Australian National University, Building 32 North Road, ACT 0200, Australia
2
Department of Electronic Materials Engineering, Research School of Physics and Engineering, Australian National University,
ACT 0200, Australia
Received 23 June 2014, revised 1 August 2014, accepted 6 August 2014
Published online 12 August 2014
Keywords ion implantation, boron, annealing, oxidation, carrier recombination, silicon solar cell emitters, sheet resistance
*
Corresponding author: e-mail tom.ratcliff@anu.edu.au, Phone: +612 6125 0078
© 2014 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim
1 Introduction The use of ion implantation for the
formation of heavily doped regions in silicon solar cells of-
fers significant process simplification compared with tradi-
tional diffusion-based processes, especially for advanced
Si solar cell structures that require patterned doping such
as interdigitated back contact cells [1]. The application of
ion implantation in industrial Si solar cell manufacturing
has also been shown to yield improved uniformity and con-
trol [2]. Following implantation, high temperature process-
ing is required to electrically activate dopant atoms and re-
pair implantation damage. However, secondary defects are
likely to form during annealing and may cause increased
Shockley–Read–Hall recombination of minority carriers
reducing the overall conversion efficiency of the device.
For boron implantation, defects such as dislocation loops
and boron-interstitial clusters have been identified as pos-
sible causes of high recombination [3, 4].
Boron-interstitial clusters (BICs) are comprised of
electrically inactive boron atoms and silicon interstitials
and can form at concentrations below the boron solid solu-
bility limit [5]. Extrinsic dislocation loops are also known
to form during annealing of Si that has been implanted
beyond a critical implant fluence [6, 7]. Both BICs and
dislocation loops form due to a local supersaturation of
interstitial silicon atoms resulting from implantation dam-
age.
The selection of either an oxidising or inert ambient during
high temperature annealing is shown to affect dopant activa-
tion and electron–hole recombination in boron implanted
silicon samples. Samples implanted with B at fluence be-
tween 3 × 10
14
cm
–2
to 3 × 10
15
cm
–2
are shown to have lower
dopant activation after oxidation at 1000 °C compared to an
equivalent anneal in an inert ambient. In addition, emitter re-
combination is shown to be up to 15 times higher after oxida-
tion compared with an inert anneal for samples with equiva-
lent passivation from deposited Al
2
O
3
films. The observed in-
crease in recombination for oxidised samples is attributed to
the enhanced formation of boron-interstitial defect clusters
and dislocation loops under oxidising conditions. It is also
shown that an inert anneal for 10 minutes at 1000 °C prior to
oxidation has no significant impact on sheet resistance or re-
combination compared with a standard oxidation process.
J
0p+
as a function of sheet resistance for Al
2
O
3
passivated
samples after 1000 °C anneal for 70 minutes.