International Journal of Chemistry; Vol. 4, No. 5; 2012
ISSN 1916-9698 E-ISSN 1916-9701
Published by Canadian Center of Science and Education
35
Modified Saw Dust for the Removal of Lead Cations from Aqueous
Media
Ismail Abbas
1
, Jinane K. Chaaban
2
& Iyad Karamé
3
1
Chemistry Department, Faculty of Science, Beirut Arab University, Tripoli, Lebanon
2
Faculty of Sciences, Lebanese University, Beirut, Lebanon
3
Department of Chemistry, Lebanese University, Beirut, Lebanon
Correspondence: Ismail Abbas, Chemistry Department, Faculty of Science, Beirut Arab University, Tripoli
11-5020, Lebanon. Tel: 961-360-1140. E-mail: i.abbas@bau.edu.lb
Received: June 8, 2012 Accepted: June 16, 2012 Online Published: September 20, 2012
doi:10.5539/ijc.v4n5p35 URL: http://dx.doi.org/10.5539/ijc.v4n5p35
Abstract
Saw dust modified with chloroethylacetate was prepared. The product was used as an extracting agent for the
solid-phase extraction of lead cations from aqueous media. The uptake performance of modified saw dust (MSD)
for removal of Pb(II) cations was investigated using batch method. The influences of some experimental
parameters like initial concentration of the cation, extraction time, concentration of the saw dust, pH and
temperature were studied. Three adsorption isotherms [Langmuir, Freundlich and Dubinin-Redushkevish (D-R)]
were used to analyze the equilibrium data. The sorption capacity of modified saw dust was found to be 78.1 mg/g
at 298 K from 164 mg/l aqueous solution of lead cation. The mean free energy calculated from D-R model was
found to be 15.81 KJ/mol, indicating that chemisorption is involved in the extraction process. The removal of lead
cation does not change with increasing temperature. The present method has been compared with the previous
methods.
Keywords: modified sawdust, Lead Cation, extraction, adsorption isotherm
1. Introduction
Rapid industrialization and poor effluent treatment processes in many industries have led to a substantial lowering
of water quality that is fed to water bodies. Presence of heavy metals is one of the many factors that lower water
quality. The heavy metals cause adverse effects on health, increase environmental toxicity and affect the aesthetic
quality of the water (Parab, Joshi, Shenoy, Lali, Sarma, & Sudersanan, 2008). The removal of heavy metal in an
effective manner from water and wastewater is, thus, ecologically very important. Common cleaning methods for
the removal of heavy metal comprise membrane separation (Chakravarti, Chwodhury, Chakraborty, Chakraborty,
& Mukherjee, 1995 ), electrochemical precipitation (Kongsricharoern & Polprasert, 1996), emulsion per traction
(Ortiz, Roman, Corvalan, & Eliceche, 2003), ion exchange (Trgo, Peric, & Medvidovic, 2006), preconcentration
(Hirata, Honda, & Kumamru, 1989), fertilization (Mandaoker, Dharmadhikari, & Dara, 1994) and adsorption
(Danil de Namor & Abbas, 2010 ; Bhattacharya, Naiya, Mandal, & Das, 2008). These methods differ with respect
to cost, complexity and efficiency.
Lead(II) is a well known highly toxic metal considered as a priority pollutant. It directly enters the water bodies
through the effluent discharges including battery, paper and pulp, mining, electroplating, lead smelting and
metallurgical finishing industries and caused a marked increase in concentrations. In most countries, lead(II) level
of water is limited with the value of 0.05 mg/l. It causes various types of acute and chronic disorders. The safe and
effective disposal of Pb(II) containing waste water is a challenging objective for industries because cost effective
treatment alternatives are not readily available. A number of adsorbents such as activated carbon (Reed,
Arunachalam, & Tomes, 1994), sargassum (K. Park, M. Park, Jang, E. Kim, & Y. Kim, 1999), chitosan (Inoue,
Ohto, Yoshizuka, Yamaguchi, & Tanaka, 1997), metal oxide gel (Shubha, Raji, & Anirudhan, 2001), saw dust
(Raji, Shubha, & Anirudhan, 1997), humus-boehmite complex (Abraham & Anirudhan, 2001), animal bone
powder and ceramics (Abdel-Halim, Shehta, & El-Shahat, 2003) have been used for lead(II) removal. The idea of
using various agricultural products and by-products for the removal of heavy metal from solution has been
investigated by number of authors (Low, Lee, & Liew, 2000). Natural materials that are available in large