© 2011 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim 343
Biotechnol. J. 2011, 6, 343–356 DOI 10.1002/biot.201000316 www.biotechnology-journal.com
1 Introduction
The yeast Saccharomyces cerevisiae is a widely
used model organism for studying eukaryal cellu-
lar and molecular principals [1]. This yeast is also
an industrial workhorse used for the production of
fuels, chemicals, food ingredients and pharmaceu-
ticals [2–4]. It is particularly well known for its role
as a cell factory for bioethanol production, where
its high ethanol tolerance allows for efficient pro-
duction, reaching very high titers. Also a number of
recombinant proteins (i.e., hormones and vaccines)
are being commercially produced by S. cerevisiae,
and here efficient protein production, folding and
secretion are of major importance [5]. There is also
much interest in exploiting yeast as a production
Research Article
Heterologous production of polyunsaturated fatty acids
in Saccharomyces cerevisiae causes a global transcriptional
response resulting in reduced proteasomal activity and
increased oxidative stress
Rawisara Ruenwai
2,3
, Andrea Neiss
1
, Kobkul Laoteng
4
, Wanwipa Vongsangnak
1
, Arastoo Badoei Dalfard
1
*
,
Supapon Cheevadhanarak
2,3
, Dina Petranovic
1
and Jens Nielsen
1
1
Department of Chemical and Biological Engineering, Chalmers University of Technology, Gothenburg, Sweden
2
School of Bioresources and Technology, King Mongkut’s University of Technology Thonburi, Bangkok, Thailand
3
Pilot Plant Development and Training Institute, King Mongkut’s University of Technology Thonburi, Bangkhuntien, Bangkok,
Thailand
4
Biochemical Engineering and Pilot Plant Research and Development Unit, National Center for Genetic Engineering and
Biotechnology, National Sciences and Technology Development Agency at King Mongkut’s University of Technology Thonburi,
Bangkhuntien, Bangkok , Thailand
Due to their health benefits there is much interest in developing microbial processes for efficient
production of polyunsaturated fatty acids (PUFAs). In this study we co-expressed Mucor rouxii Δ
12
-
and Δ
6
-desaturase genes in Saccharomyces cerevisiae, which resulted in a yeast strain that accumu-
lated linoleic acid and γ-linolenic acid in the different lipid species. Additionally, the strain contained
higher levels of phospholipids and lower levels of ergosterol than the reference strain. Integrated
analysis of the transcriptome revealed decreased expression of genes involved in ergosterol biosyn-
thesis, but more unexpectedly it also pointed towards attenuated activity of the ubiquitin-protea-
some system and a reduced oxidative stress response. In vitro and in vivo measurements showed
reduced levels of all three proteasomal activities and also increased levels of reactive oxidative
species in the PUFA-producing strain. Overall our results clearly show that PUFAs in yeast can be
detrimental for several key cellular pathways, such as the oxidative stress response and proteaso-
mal activity, suggesting that the membrane composition is of vital importance for these processes.
Keywords: Desaturase · Lipid biosynthesis · PUFAs · yeast · Stress response
Correspondence: Professor Jens Nielsen, Department of Chemical and
Biological Engineering, Chalmers University of Technology,
SE-412 96 Gothenburg, Sweden
E-mail: nielsenj@chalmers.se
Fax: +46-31-772-3801
Abbreviations: AZE, L-azetidine-2-carboxylic acid; GLA, γ-linolenic acid;
HNE, 4-hydroxy-2-nonenal; LA, linoleic acid; PUFAs, polyunsaturated fatty
acids; ROS, reactive oxidative species; UPS, ubiquitin-proteasome system
Received 21 September 2010
Revised 2 November 2010
Accepted 10 November 2010
Supporting information
available online
* Current address: Department of Biology, Faculty of Science, Shahid
Bahenar University of Kerman, Kerman, Iran