GEOLOGY, August 2011 735
INTRODUCTION
Cryogenian glaciations (750–635 Ma) were
more severe than any subsequent events and
may have recorded the most extreme climate
changes in Earth history (e.g., Hoffman and Li,
2009). Anomalously low δ
18
O values of -11‰
to -4‰ reported for Neoproterozoic igneous
zircons in ultrahigh-pressure (UHP) eclogite
facies metamorphic rocks in the Dabie-Sulu
orogenic belt of central-east China (Zheng et al.,
2008, and references therein) were often inter-
preted as representing primary oxygen isotope
compositions of Neoproterozoic rift magma-
tism of the northern margin of the South China
Block, and genetically linked to Neoproterozoic
glaciations (e.g., Zheng et al., 1998, 2004, 2007,
2008; Rumble et al., 2002).
A glaciation origin for low-δ
18
O magmas
requires magmatic rocks to acquire their oxy-
gen isotope signatures through hydrothermally
driven meteoric water under conditions of a
cold climate, such as an ice age, or through the
involvement of water from melting of glacial
ice below the base of a continental ice cap (e.g.,
Rumble et al., 2002; Zheng et al., 2008). In other
words, the glaciation origin model predicts that
Neoproterozoic magmas should display sharp
oxygen isotope shifts corresponding to the onset
of ice ages. However, in-situ zircon oxygen and
U-Pb analyses of metamorphic rocks in the
Dabie Shan orogenic belt show that such low-
δ
18
O magmatic zircons started to appear from
ca. 810 Ma (Chen et al., 2003), significantly ear-
lier than the Chang’an glaciation (no older than
725 Ma; Zhang et al., 2008; Hoffman and Li,
2009), making such a link tenuous. In addition,
except for the study of Chen et al. (2003), all
the zircon oxygen isotope data from the Dabie
Shan orogenic belt were acquired through bulk
analysis (e.g., Zheng et al., 1998, 2004, 2007,
2008; Rumble et al., 2002), which tends to pro-
duce mixed results between zircon cores and
rims, and thus does not discriminate between
magmatic and UHP metamorphic signatures.
Whole-rock primary oxygen isotope composi-
tions of Precambrian igneous rocks can be dif-
ficult to determine because they are often reset
by post-magmatic alteration. Even in relatively
retentive minerals, such as quartz, postmagmatic
alteration and recrystallization can obscure mag-
matic signatures (e.g., Valley and Graham, 1996).
Also, most low-δ
18
O magmas were probably
eroded away by younger geological processes
due to their shallow genesis (e.g., Bindeman,
2008). Although eroded igneous rocks are lost
from the rock record, their depleted
18
O signa-
tures could be preserved in sedimentary basins
by refractory minerals, such as zircon. Due to
its extremely slow rate of oxygen diffusion and
high closure temperature, zircon is insensitive to
hydrothermal alteration and fractional crystal-
lization during cooling, and can therefore retain
its primary oxygen isotope composition from the
time of crystallization (e.g., Valley, 2003).
The Nanhua Rift is the largest failed continen-
tal rift basin in the South China Block and has
some of the best-preserved sedimentary and vol-
canic rocks related to the breakup of the supercon-
tinent Rodinia and the Neoproterozoic Snowball
Earth (e.g., Wang and Li, 2003; Li et al., 2008)
(Fig. 1A). Four fine-grained sedimentary samples
were collected from Cryogenian sedimentary
sequences in the Nanhua Rift basin (Figs. 1A and
1B) for zircon age and oxygen isotope determina-
tions, including one tuff sample (08SC31, grain
size is slightly smaller than that of typical silt-
stone) and three siltstone samples (08SC07 and
08SC11are tuffaceous siltstones and 08SC74 is
siltstone). We analyzed these samples by micro-
analytical techniques using a Cameca IMS-1280
secondary ion mass spectrometer (SIMS), which
permits rapid, high-precision in-situ analysis of
oxygen isotopes in zircon (e.g., Kita et al., 2009;
Li et al., 2010a). High analytical precision and
spatial resolution made it possible to identify pre-
viously undetectable variations in oxygen isotope
composition, thus providing new insights into the
causes for the large-scale
18
O-depletion event in
the Neoproterozoic.
RESULTS
Zircon oxygen isotope compositions are pre-
sented in Figures DR2 and DR3 and in the GSA
Data Repository
1
. The data have been divided
Geology, August 2011; v. 39; no. 8; p. 735–738; doi:10.1130/G31991.1; 3 figures; Data Repository item 2011223.
© 2011 Geological Society of America. For permission to copy, contact Copyright Permissions, GSA, or editing@geosociety.org.
*E-mail: X.Wang3@curtin.edu.au.
Nonglacial origin for low-δ
18
O Neoproterozoic magmas in the South
China Block: Evidence from new in-situ oxygen isotope analyses
using SIMS
Xuan-Ce Wang
1, 2, 3
*, Zheng-Xiang Li
2
, Xian-Hua Li
1
, Qiu-Li Li
1
, Guo-Qiang Tang
1
, Qi-Rui Zhang
1
, and Yu Liu
1
1
State Key Laboratory of Lithospheric Evolution, Institute of Geology and Geophysics, Chinese Academy of Sciences, P.O. Box
9825, Beijing 100029, China
2
Institute for Geoscience Research, Department of Applied Geology, Curtin University, GPO Box U1987, Perth, WA 6845, Australia
3
School of Earth and Environment, the University of Western Australia, Crawley, WA 6009, Australia
ABSTRACT
Low-δ
18
O signatures in supracrustal rocks have been used as geochemical proxies for cold
paleoclimates, e.g., glaciations. Unusual low-δ
18
O values found in Neoproterozoic igneous
rocks in parts of the South China Block have thus been genetically linked to Neoprotero-
zoic glaciation events. However, we report here new oxygen isotope compositions from Neo-
proterozoic magmatic zircons in central southern China using in-situ techniques that argue
against such an interpretation. Our results show that (1) low-δ
18
O magmatic zircons started
to appear in the South China Block from ca. 870 Ma, coinciding with the tectonic switching
from Sibao orogenesis to postorogenic extension, which occurred more than 150 m.y. prior to
the first glaciation event. The most abundant low-δ
18
O magmatic zircons have ages of 800–
700 Ma. (2) The 830–700 Ma magmatic zircons are characterized by their bimodal nature of
oxygen isotope compositions, i.e., mantle-like δ
18
O values (+4.4‰ to +5.8‰) and high-δ
18
O
values (+9.3‰ to +10.8‰). (3) A sharp temporal change in maximum zircon δ
18
O values in
the South China Block coincided with the onset of continental rifting and the possible arrival
of a plume head. (4) No negative δ
18
O zircons have been identified in this study, contrary to
previous studies. These features strongly argue against a glaciation origin for low to negative
δ
18
O values in Neoproterozoic magmatic zircons from southern China. We propose that two
stages of high-temperature water-magma interaction during plume-driven magmatism and
continental rifting best explain the low-δ
18
O magmas. The most important implication of this
study is that formation of such low-δ
18
O magmatic zircons was not necessarily related to gla-
cial events and should not be used as a geochemical proxy for a cold paleoclimate.
1
GSA Data Repository item 2011223, secondary
ion mass spectrometer zircon oxygen and U-Pb ana-
lytical methods and data, is available online at www
.geosociety.org/pubs/ft2011.htm, or on request from
editing@geosociety.org or Documents Secretary,
GSA, P.O. Box 9140, Boulder, CO 80301, USA.