6
Cellular and Molecular
Biology
Original Research
Puriication and characterization of polyphenol oxidase from corn tassel
R. Gul Guven¹
*
, N. Aslan¹, K. Guven², F. Matpan Bekler
3
, O. Acer²
1
Science Teaching Section, Education Faculty, Dicle University, Diyarbakir, Turkey
2
Molecular Biology and Genetics Departement, Science Faculty, Dicle University, Diyarbakir, Turkey
3
Biology Departement, Science Faculty, Dicle University, Diyarbakir, Turkey
Abstract: In this study, polyphenol oxidase (PPO) from corn tassel was extracted and partially puriied through (NH
4
)
2
SO
4
precipitation and gel
iltration chromatography. Optimal temperatures for subsrates catechol and 4-methyl catechol were 40 °C and 30 °C, respectively. The optimal
pH values were 8.0 for catechol and 6.0 for 4-methyl catechol. Catechol was the most suitible substrate (Km: 3.48 mM, Vmax: 1.0 Abs./ min.).
The moleculer mass of PPO was determined as 158 kDa. In this work, sodium azide, ethylenediaminetetraacetic acid (EDTA) and sodium dode-
cyl sulfate (SDS) were found to inhibit the enzyme activity as 26.6 %, 22.2 % and 12.2 % ratio, respectively. Besides, the effects of carbohydrates
such as sucrose, fructose, ribose and glucose on PPO activity were investigated. The enzyme was found to be activated 17 % by fructose and
ribose, 16 % by glucose and 4 % by sucrose.
Key words: Corn tassel , polyphenol oxidase,characterisation, substrate speciity, inhibition.
Introduction
Polyphenol oxidases (PPO), belong to a set of cop-
per containing metalloenzymes that are members of
oxidoreductases that catalyze the oxidation of a wide
range of phenolic compounds by utilizing molecular
oxygen (1). Polyphenol oxidase is widely distributed
among higher plants, which is an enzyme responsible
for hydroxylation of monophenols to form o-diphenols
and their further oxidation to colored and highly reac-
tive o-quinones. PPO is well known to be the principal
enzyme involved in enzymatic browning. Particularly,
when a plant gets a bruise, cut or damage, the enzyme
leads to the oxidation of typical phenolic compounds to
form a polymer structure, resulting in protection of the
plant against microorganisms or insects (2). This pro-
cess causes enzymatic browning of fruits and vegetables
which is undesirable in food technology as it results in
loss of quality (3, 4, 5).
Corn (Zea mays L.) is one of the most widely planted
crops over the world and the world production was es-
timated to be 471 million tons (6). Corn tassels are a
waste part of the plant, which can be processed to pro-
duce valuable products such as volatile oils (7), the la-
vonol glycosides of kaempferol, isorhamnetin and quer-
cetin (8) and lipids (9). Corn tassel (CT) is mainly seen
as waste by corn processing industry. Since it contains a
variety of active ingredients, such as lavonoid, alkaloid,
allantoin, pentosan, inositol, polysaccharide, vitamin K,
vitamin C, several kinds of organic acids, and sterols,
CT may well serve as an inexpensive herbal drug (10).
Therfore, it is of importance to characterise the enzymes
such as PPO leading to loss of quality in corn tassel.
PPO has been isolated and puriied from various
sources, such as Turkish tea leaf (11), strawberry (12)
,ispir sugar bean (13), persimmon (14), and Jackfruit
(15), Ataulfo mango (16) and its properties have been
extensively studied. To our best knowledge, there is no
data in literature on the puriication and characteriza-
tion of PPO from corn tassel. The main objectives of
the present study are to characterize PPO puriied from
corn tassel, to determine its kinetic and characteristic
properties, as well as investigating the effect of some
activators and inhibitors on the enzyme activity to elu-
cidate the mechanism of its inhibition by selected che-
mical compounds.
Materials and Methods
Materials and reagents
The corn tassel was obtained from a local market
Diyarbakir City, Turkey and stored in 4°C until used.
Catechol was purchased from Merck (Darmstadt, Ger-
many). Ammonium sulphate, 4-methylcatechol, Se-
phadex G-100 gel iltration resin, polyethylene glycol
(PEG), citric acid and all chemicals for electrophoresis
studies were purchased from Sigma Chem. Co. All che-
micals used in this study were of analytical grade.
Preparation and extraction of polyphenoloxidase
(PPO) from corn tassel
Corn tassel (14.50 grams) obtained from the local
market was homogenized in the extraction solution 100
ml of 0.1 M phosphate buffer containing 4 % PEG at pH
6.5 and 10 mM ascorbic acid by using a blender. The
crude extract samples were centrifuged at 10.000 g for
20 min at 4 ºC. The homogenate was iltered through
double layered ilter paper. Solid ammonium sulphate
(NH
4
)
2
SO
4
was slowly added to the supernatant to get
80 % (NH
4
)
2
SO
4
saturation under cold conditions. After
1 h, centrifugation was carried out at 15.000 g for 30
min to separate the precipitated proteins. The precipi-
Received June 28, 2016; Accepted November 03, 2016; Published
November 30, 2016
* Corresponding author: Assoc. Prof. Reyhan Gul Guven, Dicle University,
Education Faculty, Science Teaching Section, Diyarbakir, Turkey. Email:
rgguven@dicle.edu.tr
Copyright: © 2016 by the C.M.B. Association. All rights reserved.
Gul Guven et al. Cell. Mol. Biol.2016, 62 (13): 6-11
ISSN: 1165-158X
doi: 10.14715/cmb/2016.62.13.2