Vol 10, Issue 3, 2017
Online - 2455-3891
Print - 0974-2441
GREEN SYNTHESIS OF SUPERPARAMAGNETIC IRON OXIDE NANOPARTICLE FROM
FICUS CARICA FRUIT EXTRACT, CHARACTERIZATION STUDIES AND ITS APPLICATION ON DYE
DEGRADATION STUDIES
THARUNYA P
1
, SUBHA V
1
, KIRUBANANDAN S
1
*, SANDHAYA S
2
, RENGANATHAN S
1
Centre for Biotechnology, Anna University, Chennai, Tamil Nadu, India.
2
Department of Biotechnology, VIT University, Vellore, Tamil Nadu,
India. Email: skirubanandan80@gmail.com
Received: 05 October 2016, Revised and Accepted: 22 December 2016
ABSTRACT
Objective: The synthesis of nanoparticles (NPs) has become a matter of great interest in recent times due to their various advantageous properties
and applications in a variety of fields. Metal NPs are being increasingly used in many sectors, and there is growing interest in the biological and
environmental safety of their production.
Methods: In this study, iron oxide NPs (Fe
3
O
4
-NPs) were synthesized from fruits of Ficus carica using a rapid, single step and completely green
biosynthetic method by reduction of ferrous sulfate solution with F. carica ethanolic extract. The prepared Fe
3
O
4
-NPs were investigated by X-ray
diffraction, Fourier transform infrared spectroscopy, and ultraviolet-visible spectroscopy.
Results: The report emphasizes the effect of superparamagnetic Fe
3
O
4
-NPs on the degradation rate of hazardous dyes acid blue.
Conclusion: To conclude, Fe
3
O
4
-NPs were prepared from fruits of F. carica using a rapid, single step and completely green biosynthetic method by
reduction of ferrous sulfate solution with F. carica ethanolic extract.
Keywords: Ficus carica, Ethanolic extract, Reduction, Ferrous sulfate, Superparamagnetic iron oxide nano particles, Dye degradation.
INTRODUCTION
Nanotechnology is a multidisciplinary branch of science that
encompasses numerous fields of science and technology, including
biomedicine, pharmaceutics, environmental science, and others [1].
The use of nanoparticle [NP] materials offers advantages due to their
unique size and physicochemical properties. NPs are clusters of atoms
in the size range of 1-100 nm. The control of the monodisperse size of
NP is very important because the properties of the nanocrystals strongly
depend on the dimension of the NPs. One of the most commonly-used
nanoscale materials is magnetic NPs (MNPs): A type of core/shell NP
structure that consists of a magnetic core encapsulated in an organic or a
polymeric coating. Without a coating, MNPs have hydrophobic surfaces
with large surface-to-volume ratios and a propensity to agglomerate [2].
Iron oxide NPs (Fe
3
O
4
-NPs) have attracted intensive research
interest because of their important applications in cancer therapy,
drug delivery, magnetic resonance imaging (MRI), and wastewater
treatment [3]. Superparamagnetic Fe
3
O
4
-NPs with appropriate surface
chemistry can be used for numerous in vivo applications, such as MRI
contrast enhancement, tissue repair, and immunoassay, detoxification
of biological fluids, hyperthermia, drug delivery, and cell separation [4].
The biosynthesis of Fe
3
O
4
-NPs of different sizes and shapes has been
reported using bacteria [5,6] and plant extract [7]. The stability of iron
NPs against aggregation can be improved by imparting electrostatic
repulsion, applying organic surfactants, or through the use of capping
agents [8]. In recent times, sources of dye contamination have
expanded from textile industries to food, paper, printing, cosmetic,
and pharmaceutical companies [9]. When these dyes are not treated
properly, they get accumulated in the environment and become a threat
to the ecosystem. These non-treated dyes are potentially carcinogenic,
mutagenic and genotoxic, example of such dyes include Acid Red 26,
Direct Blue 6, Direct Black 38, etc. Abatement of dyes is a required part
of wastewater treatment. Nanotechnology has been extended to the
wastewater treatments in the recent years. Due to high surface area
silver NPs exhibits an enhanced reactivity [10,11].
Ficus carica is known to contain polyphenols and flavonoids that
act both as a reducing agent and a capping agent. Its fruit, root, and
leaves are used in traditional medicine to treat various ailments such
as gastrointestinal (colic, indigestion, loss of appetite, and diarrhea),
respiratory (sore throats, coughs, and bronchial problems), and
cardiovascular disorders and as anti-inflammatory and antispasmodic
remedy.
A wide variety of methods have been reported in for the synthesis of
Fe
3
O
4
NPs such as microemulsion technique [12], electrochemical
route [13], hydrothermal process [14], sonochemical method [15], and
co-precipitation method [16]. Nowadays, synthesis of Fe
3
O
4
-NPs using
phytochemicals has attracted much attention due to their simplicity,
environmental benignity, and low cost.
Dyes are a major class of synthetic organic compounds released by
many industries such as paper, plastic, leather, food, cosmetic, textile,
and pharmaceutical industries [17,18]. The synthesis and applicability
of the Fe
3
O
4
-NPs in the effective removal of acid blue have been reported.
The main objective of this study is to test the applicability of Fe
3
O
4
NPs
as a catalyst in the removal of acid blue dye. Photocatalytic degradation
of acid blue was conducted using Fe
3
O
4
NP as a catalyst in the presence
of sunlight.
METHODS
Sample collection
Fig fruits were collected from Anna University, ACT Campus, Chennai,
Tamil Nadu, India.
© 2017 The Authors. Published by Innovare Academic Sciences Pvt Ltd. This is an open access article under the CC BY license (http://creativecommons.
org/licenses/by/4. 0/) DOI: http://dx.doi.org/10.22159/ajpcr.2017.v10i3.15538
Research Article