Au–Cu BIMETALLIC COLLOIDS PREPARED BY COCONDENSATION WITH
NONAQUEOUS SOLVENTS
Galo Ca ´rdenas T.
1
*, Marcela Gonza ´lez G.
1
, Elizabeth Salgado C.
1
, Juan Morales
2
,
and Hugo Soto Z.
2
1
Departamento de Polı ´meros, Facultad de Ciencias Quı ´micas, Universidad de Concepcio ´n,
Casilla 160-C, Concepcio ´n, Chile
2
Departamento de Fı ´sica, Facultad de Ciencias Fı ´sicas y Matema ´ticas, Universidad de
Concepcio ´n, Concepcio ´n, Chile
(Refereed)
(Received October 19, 1998; Accepted December 31, 1998)
ABSTRACT
Au–Cu colloids were prepared by chemical liquid deposition (CLD). The
metals were evaporated simultaneously to yield atoms, which were solvated to
yield bimetal atom mixtures at 77 K, and upon warming, in some cases, stable
liquid colloids were formed with a narrow range of particle size. The solvents
under study were acetone, 2-butanone, 2-propanol, 2-methoxyethanol,
2-ethoxyethanol, diglyme, THF, and DMF. The particle size of the bimetallic
colloids ranged from 21 to 48 Å. The films or powders were prepared by direct
evaporation of the solvents from bimetallic colloids. Microanalysis demon-
strated that these films contained carbon and hydrogen residues. Infrared
spectra showed that hydrocarbon residues were present in the films. Thermal
studies demonstrated the low stability of the Au–Cu films. Two or three
decomposition temperatures were observed in the thermograms. In most of the
films, a total weight loss of 10 –15%, at 550°C, was registered. © 2000 Elsevier
Science Ltd
KEYWORDS: A. alloys, A. amorphous materials, A. nanostructures, A. thin
films, B. vapor deposition, A. semiconductors
*To whom correspondence should be addressed.
Materials Research Bulletin, Vol. 34, Nos. 12/13, pp. 1911–1919, 1999
Copyright © 2000 Elsevier Science Ltd
Printed in the USA. All rights reserved
0025-5408/99/$–see front matter
PII S0025-5408(99)00199-3
1911