Open Journal of Organic Polymer Materials, 2014, 4, 29-36
Published Online January 2014 (http://www.scirp.org/journal/ojopm )
http://dx.doi.org/10.4236/ojopm.2014.41005
OPEN ACCESS OJOPM
Synthesis of Poly(APP-co-EGDMA) Particles Using
Monomers Derived from Cashew Nut Shell Liquid for the
Removal of Cr(III) from Aqueous Solutions
Joseph Wilson
1
, Joseph Yoeza Naimani Philip
2
, James Epiphan Gabriel Mdoe
2
1
Department of Chemistry, St. John’s University of Tanzania, Dodoma, Tanzania
2
Chemistry Department, University of Dar es Salaam, Dar es Salaam, Tanzania
Email: james_mdoe@yahoo.co.uk
Received November 15, 2013; revised December 15, 2013; accepted December 22, 2013
Copyright © 2014 Joseph Wilson et al. This is an open access article distributed under the Creative Commons Attribution License,
which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited. In accor-
dance of the Creative Commons Attribution License all Copyrights © 2014 are reserved for SCIRP and the owner of the intellectual
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ABSTRACT
This work was aimed at synthesizing Cashew Nut Shell Liquid (CNSL) based polymer particles for adsorption of
Cr(III) ions from aqueous solutions. Natural CNSL was used as a starting material in synthesizing amino penta-
decylphenols (APP). This was achieved through isolating anacardic acid from the CNSL via calcium anacardate
procedure, followed by hydrogenation of the alkenyl side chains, and subsequently decarboxylating the product
to form 3-pentadecylphenol, which was then nitrated and reduced to a mixture of APP. APP were co-polyme-
rized with ethylene glycol dimethacrylate (EGDMA) to form poly(APP-co-EGDMA) particles. The chemical
structures of the synthesized compounds were confirmed by Fourier Transform IR and 1H-NMR. The co-poly-
mer particles were characterized by Scanning Electron Microscopy (SEM) to establish their morphological
properties. The prepared co-polymer particles were found to have -NH loading of 46 mmol/g and a maximum
adsorption capacity for Cr(III) ions of 16 mg per g of dry polymer particles. The spent polymer particles were
recoverable and reusable.
KEYWORDS
Cashew Nut Shell Liquid (CNSL); Amino Pentadecylphenols (APP); Poly(APP-co-EGDMA)
1. Introduction
Environmental pollution by heavy metals is a widespread
problem nowadays due to increased anthropogenic activ-
ities. In most cases, the pollution load ends into water
bodies thus threatening not only aquatic organisms, but
also the quality of water for domestic uses. Pollution
from heavy metals is one of the most serious environ-
mental problems due to the fact that they bio-accumulate
causing adverse effects to living organisms [1]. In view
of this, their removal from industrial discharged effluents
becomes an absolute necessity.
Chromium is one of the heavy metals known to be
toxic to humans and aquatic life. Various industrial efflu-
ents from pigments, electroplating, dying, canning, textile,
leather tanning, paint and steel industries contain substan-
tial amounts of chromium. In general, these industrial
effluents contain both Cr(III) and Cr(VI) ions. However,
it is well established that Cr(III) is not as toxic as Cr(VI).
Yet under suitable conditions, Cr(III) can readily be oxi-
dized to Cr(VI) [2], thus underlying the importance of re-
stricting its accumulation in the environment. Further-
more, excessive buildup of Cr(III) ions can affect the
ecology of the environment as well as inhibiting various
enzyme systems in living organisms [3,4]. Long term ex-
posure to Cr(III) is also known to cause cancer and aller-
gic skin reactions [5].
The importance of minimizing the amount of Cr(III)
ions in industrial effluents and other sources has led to
the development of a number of removal methods. The
commonly used methods for removing such metal ions
from aqueous waste include precipitation, lime coagula-
tion, semi-sedimentation, electro-dialysis, chemical reac-