American Journal of Environmental Science, 2012, 8 (4), 412-416
ISSN: 1553-345X ©2012 Science Publication
doi:10.3844/ajessp.2012.412.416 Published Online 8 (4) 2012 (http://www.thescipub.com/ajes.toc)
412
Science Publications AJES
COMPARISON OF TWO ANALYTICAL TECHNIQUES FOR
LEAD DETERMINATION IN SOILS AND MOSSES SAMPLES
1
Albert Maxhuni,
2
Pranvera Lazo and
1
Musaj Paqarizi
1
Department of Chemistry, Faculty of Natural Sciences, University of Prishtina, Kosovo
2
Department of Chemistry, Faculty of Natural Sciences, University of Tirana, Albania
Received 2012-03-07; Revised 2012-06-21; Accepted 2012-06-21
ABSTRACT
The aim of this study was to compare the results of the lead levels obtained by two different techniques in
the soil and mosses samples taken from the entire territory of the Republic of Kosovo. The atmospheric
deposition of lead through the biomonitoring technique was done for the first time in Kosovo by using
quartz tube flame Atomic Absorption Spectroscopy (AAS) and furnace AAS. The analytical results
obtained by both techniques were very close to each other for the concentration of lead up to 0.15 mg kg
-1
.
Mosses were used as bioindicators due to the purpose that they take the food from the rainfall and
atmospheric dust. Two types of terrestrial mosses (Pseudosclerpodium purum and Hypnum cupressiforme)
and the soil, collected in June-July 2011 at 25 sites evenly distributed over the whole region of Kosovo,
were used in this study. The lead concentration varies from ~ 11-416 mg kg
-1
in the soil and from ~ 3-50
mg kg
-1
, DW in mosses, depending on the pollution zone. From the obtained results, we conclude that the
lead levels are higher at the sampling positions near the polluted area of industry and heavy traffic.
Keywords: Atmospheric deposition, trace elements, lead, air pollution, soil pollution, quartz tube technique
1. INTRODUCTION
The method of utilizing mosses as bioindicators was
applied more than three decades ago (Rühling and Tyler
1973) and now is a widely accepted method for
estimation of atmospheric depictions of metals (Rühling
and Steinnes 1998; Harmens et al., 2004). Mosses have
only a rudimentary root system and take up elements
from the atmosphere. This method has as advantage the
simple sample collection and relative easiness of analysis
compared to other techniques used for this purpose. The
results from the survey of mosses analyzes allow
examination of temporal and spatial distribution of
different inorganic and organic pollutants and also the
identification of the particular areas that are highly
polluted from this metal due to the long-range transport
and other local sources.
The technique using moss as bioindicators for
assessing heavy metal distribution had been
successfully applied by different groups (Ermakova et
al., 2004; Barandovski et al., 2008).
Pb in soil represents a major environmental and human
health concern due to their high toxicity, low
biodegradability and cumulative tendency.
In the Republic of Kosovo so far there is no
monitoring program that deals with the traces metals
determination in the atmosphere. From the results of
previous studies (Borgna et al., 2009) it was pointed out
that some areas are contaminated with elevated levels of
lead and other heavy metals in Kosovo. The primary goal
is to have an overview regarding the distribution of heavy
metals from atmospheric deposition from air and soil
pollution. Aiming to achieve a low cost analysis, the
levels of lead in the moss samples were determined by
two different atomic absorption spectrophotometry
techniques: A) quartz tube flame AAS; b) graphite
furnace AAS; and the results were compared.
2. MATERIALS AND METHODS
2.1. Study Area
The Republic of Kosovo, located in the central part
of Balkan, is a landlocked country with an area of 10,887
km
2
with approximately 63% of the territory in
mountainous regions. The country’s population is around
2 million people. The major urban areas are Pristina,
Mitrovica, Prizeren, Peja, Gjakova, Gjilan and Podujeva.