CHEMIJA. 2008. Vol. 19. No. 2. P. 9–12
© Lietuvos mokslų akademija, 2008
© Lietuvos mokslų akademijos leidykla, 2008
Application of immobilized citrate lyase in a
bioanalytical system for determination of citrates
Asta Kaušaitė
1
,
Almira Ramanavičienė
1, 2
,
Arūnas Ramanavičius
1, 2
*
1
Center of Nanotehnology
and Materials Science,
Faculty of Chemistry,
Vilnius University,
Naugarduko 24,
LT-03225 Vilnius, Lithuania
2
Laboratory of Immunoanalysis
and Nanotechnology,
Institute of Immunology
of Vilnius University,
Molėtų pl. 29,
LT-08409 Vilnius, Lithuania
* Corresponding author. E-mail: arunas@imi.lt
A bioanalytical protocol based on the enzymatic-spectrophotometric micro-method for de-
termination of citrate with immobilized citrate lyase (CL) is described. In the design of this
spectrophotometric bioanalytical system, L-malate dehydrogenase (L-MDH), oxaloacetate de-
carboxylase (OACD) and L-lactate dehydrogenase (L-LDH) were applied as a biological recogni-
tion system. Immobilized CL catalysed the conversion of citrate to oxaloacetate and acetate. In
the presence of the enzymes L-MDH and L-LDH, oxaloacetate and its decarboxylation product
pyruvate were reduced to L-malate and L-lactate, respectively. he concentration of citrate is
stoichiometric to the concentration of nicotinamide adenine dinucleotide (NADH) formed in
enzymatic reaction. NADH was determined by means of its light absorbance at 340 nm. he
maximal diference in light absorbance was detected when CL had been immobilized on porous
carbon. If CL had been immobilized on wool ibres or carbon rod the absorbance diference
ater 360 min was almost 2 times and 3.2 times lower, respectively, as compared with the re-
sults observed when CL had been immobilized on porous carbon. he method proposed here
has several advantages if compared with the technique based on dissolved CL. Moreover, this
method allows achieving a higher rate of CL-catalysed reaction and to reduce the duration of
analysis versus the previously suggested methods. We expect that this method can be employed
for determination of other analytes by applying the corresponding enzymes in the design of the
bioanalytical system.
Key words: bioanalytical chemistry, enzymatic detection, biosensors, citrate lyase, citric acid,
citrate
INTRODUCTION
An important ield of analytical chemistry is determination of
biologically active substrates. Here, the most promising are bio-
analytical systems that are based on immobilized enzymes [1]
or some ainity exhibiting materials [2] because such systems
allow to determine a variety of biologically active analytes (e. g.,
glucose, creatine, citric acid, citrates and many others) [3]. Citric
acid and citrates are present in numerous natural products. hey
are very important intermediates in the metabolism of plants,
animals and microorganisms. In the human body, citrates are
metabolised and excreted by the kidney [4]. Citrates are prod-
ucts of normal oxidative pathways in the body of mammalians
and are normally excreted in the urine [5]. Urinary citrates play
an important role in the endogenous inhibiting of the formation
of calcium-containing kidney stones [6]. Citrates form stable
soluble complexes by chelating calcium [7], directly prevent-
ing the crystallization and precipitation of calcium-containing
compounds [8]. Moreover, citrates interact with Tamm–Horsfall
proteins and inhibit Ca-oxalate crystallization [9]. Low urinary
citrate concentrations are found in approximately half of adult
patients with renal stones [10]. Citric acid is used in the food
and beverage industry to improve and protect lavour and aro-
ma, and in cosmetics for pH adjustment. It is a component of
many pharmaceuticals and washing powders.
Determination of citric acid and citrates has become an
important item for biological luids (e. g., serum, urine, plas-
ma, seminal, sperm plasma) and foodstufs. Several methods
have been proposed for the determination of citrates based on
ion-exchange chromatography [11], high performance liquid
chromatography (HPLC) [12], capillary electrophoresis [13]
and isotachophoresis [14]. hese methods are time-consuming
procedures; besides, sample preparation is required in order to
separate citric acid from other co-existing tricarboxylic acids.
Other approaches based on conductometric or spectrophoto-
metric methods [15] sufer from selectivity as they are based on
non-speciic reactions with carboxylic acids. he above-men-
tioned selectivity problems could be potentially solved by using
a high speciicity enzyme such as citrate lyase (CL) [16–19].
Enzymatic methods allow a rapid and reliable determination of
several constituents. Enzymes are valuable analytical tools and
ofer sensitive and speciic methods for quantitative analysis;
especially useful and reliable are bioanalytical systems based
on immobilized enzymes [20]. Firstly, the procedure utilizing