International Research Journal of Engineering and Technology (IRJET) e-ISSN: 2395 -0056
Volume: 04 Issue: 02 |Feb -2017 www.irjet.net p-ISSN: 2395-0072
© 2017, IRJET | Impact Factor value: 5.181 | ISO 9001:2008 Certified Journal | Page 679
Predictive Model for Corrosion Inhibition of Mild Steel in HCl by
Crushed Leaves of Clerodendrum Splendens
Agha Inya Ndukwe
1
and C. N. Anyakwo
2
1. Department of Metallurgical Engineering Technology, Akanu Ibiam Federal Polytechnic Unwana, P.M.B. 1007,
Afikpo, Nigeria.
2. Department of Materials and Metallurgical Engineering, Federal University of Technology, P.M.B. 1526, Owerri,
Nigeria.
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Abstract - The corrosion inhibition of mild steel in 0.7M,
1.2M and 2.2M HCl by thoroughly crushed leaves of
Clerodendrum Splendens has been studied using the weight-
loss technique. The corrosion rate curves were observed to
continuously decrease with time whilst the inhibition efficiency
improved as the experimentation progressed. For the entire
study environment, the highest inhibition efficiency of 70.70%
was achieved when the thoroughly crushed leaves of
Clerodendrum Splendens were added at 45g per litre of 1.2M
HCl while the corrosion rate reduced from 0.6738mgcm
-2
h
-1
to
0.2465mgcm
-2
h
-1
. The predictive corrosion rate model was
developed using multiple regression and artificial neural
network. The prediction of the experimental corrosion rate by
the artificial neural network revealed the importance of
independent variables; (time (h), concentration of acid (M)
and quantity of crushed leaves (g)) in the prediction of the
dependent variable (Corrosion rate, CR (mgcm
-2
h
-1
). The
addition of the crushed leaves of Clerodendrum Splendens to
the hydrochloric acid induced corrosion of mild steel indicates
that the time of exposure vastly influenced the prediction of
the corrosion rate by 47.7%, followed by the quantity of
pounded leaves, 26.6% and finally the concentration of acid,
25.7%. Predictions by the artificial neural network gave a
minimal error and were closer to the experimental corrosion
rate values in comparison with the predictions by multiple
regression. The protective film formed on the mild steel
surface was analyzed by FTIR spectroscopy and Scanning
electron microscopy (SEM). The FTIR analysis indicates that
the adsorbed constituents of the crushed fresh leaves of
Clerodendrum Splendens on the surface of mild steel,
immersed at 30g per litre of 0.7M HCl for eight hours is
associated with the stretching vibrations of O–H, C≡C and C=C
bonds. The SEM image shows that corrosion was localized on
the surface of mild steel when immersed in the uninhibited
solution of 0.7M HCl but the addition of Clerodendrum
Splenden’s pounded fresh leaves at 30g per litre of 0.7M clearly
inhibited the mild steel from corrosion. The phytochemical
analysis of the leaves of Clerodendrum Splendens reveals the
presence of alkanoid, tannin, saponin, phytate, flavonoid and
phenol.
Key Words: Inhibition efficiency, Hydrochloric acid,
Corrosion rate, Clerodendrum Splendens, Artificial
eural network, Multiple regression.
1. INTRODUCTION
Corrosion is the destructive attack of a metal by
chemical or electrochemical reaction with its
environment [1]. When a metal interacts with the
environment, the tendency of the metal to revert to its
original state where it was in combination with other
elements is imminent. The overall outcome of
corrosion as acknowledged by [2] is that a metal
undergoes an electrochemical reaction as a result of its
surrounding to form a compound similar to the one
from which it was won. The destructive effect of a
metal has huge financial toll running into billions. For
instance, the total annual corrosion cost in the US rose
from $276 billion in 1998 to above $1 trillion in the
middle of 2013 and is now estimated at $1.1 trillion for
2016 [3].
The addition of an inhibitor is one of the
techniques used to prevent corrosion. Inhibitors are
substances that prevent the corrosion of metals and
alloys when added in minute quantity to the corrodent.
This may be achieved by lowering anodic or cathodic
reaction rates or both simultaneously [2]. One of such
substances often used as an inhibitor is chromate
which is toxic and carcinogenic [1]. The toxicity effect
of the known synthesized inhibitors has driven
contemporary studies towards the use of plant extracts
as anti-corrosion agents, because they are mostly
harmless.
Green inhibitors like natural products from
plant extracts and substances from other renewable
sources are of the interest of researchers who are
desirous of green chemistry or eco-friendly
technologies [4]. This research examines the leaves of
Clerodendrum Splendens as a veritable candidate for
the inhibition of mild steel in hydrochloric acid.
Clerodendrum Splendens (Verbenaceae) is a woody or
semi-woody evergreen vine or running shrub to 12ft
(3.7m) long that climbs by twining. The leaves are oval
to 7in (18cm) long and arranged in opposite pairs [5].
Inhibitors have always been considered to be
the first line of defence against corrosion in various
industries. A great number of scientific studies have
been devoted to the subject of corrosion inhibitors but