ELSEVIER Inorganica Chimica Acta 254 (1997) 213-217
Preliminary Communication
A cationic iron(III) porphyrin encapsulated between the layered structure
of MoS2. A new approach to the synthesis of an Fe-Mo-S system
Shirley Nakagaki, Antonio S. Mangrich, Fernando Wypych
Departamento de Quimica, UniversidadeFederaldo Paranti (LABEPR).C.P. 19081, CEP 81531.990 Curitiba. PR. Brazil
Received 8 July 1996;revised11 November 1996
Abstract
A new Fe-Mo-S system was obtained from the interaction of MoS2and an iron(I11) porphyrin. The products were charact~rised by X-ray
diffraction, UV-Vis and EPR spectroscopies.X-ray diffraction measurements indicated the formationof two distinct productsdepending on
the {iron porphyrin} / {single layer MoS2} ratio employed.The interlayerexpansions (Adt ~-.4A; Ad,=9 A) suggestedmono- and bi-tayer
arrangementsof the iron porphyrin into the van der Waals gaps between the host plates.
Keywords: Nanocomposites: Molybdenum disulfide complexes: Porphyrin complexes; Nitrogenase complexes: EPR spectroscopy
1. Introduction
The research field of the nanocomposites has recently
attracted considerable interest, particularly when two-dimen-
sional inorganic host lattices and polymeric organic guests
are cor~cerned [1-5]. Such systems, in which components
are mixed at the molecular level, can show hybrid physical
and ,::heroical properties derived both from the host frame-
work and the encapsulated (guest) molecules.
The interest in Fe-Mo-S systems is related to the impor-
tan~.e of biological nitrogen fixation catalysed by the
nilrogenases, a component of which, known as the Mole
protein, contains a unique Fe--Mo-S cluster believed to be
the active site for dinitrogen reduction [6,7a]. Attempts to
~ynthesize structural models of this heterometallic cluster
(the FeMoco cofactor) have produced a number of linear
and cubanc-like metal-sulfur assemblies [ 7b ]. In this work,
we introduce a new synthetic approach to an Mo-Fe-S sys-
tem. Our interest in the preparation and characterisation of a
nanocomposite consisting of the encapsulation of iron(llI)
porphyrin between the layers of MoS,, is in consequence of
the use of solid catalytic materials on heterogeneous catalysis
[8,9]. We have been able to produce nanocomposites by
interacting an iron porphyrin with single layers of the com-
mercial compound 2H-MoS2.
Layered nanocomposites derived of two-dimensional host
lattices resemble intercalation compounds; the two types of
material normally differ only in the preparation methods. In
intercalation compounds, the diffusion rate of the guest mol-
ecules into the host lattice decreases as the size of the guest
increases. As a consequence, it is not possible to prepare
intercalation compounds with organic polymers. In order to
overcome this problem, two procedures have been developed:
(i) intercalation of the monomer followed by chemical or
thermal polymerisation [1,3]; (ii) encapsulation of the
polymer by exfc!iation. This consists ofobtaining single lay-
ers of the host material, promoting the adsorption of the
polymer to the single layers and finally allowing them to re-
aggregate [4,10-12]. The second method was employed in
this work, when raeso-tetrame~hylpyfidylporphyrin iron (HI)
(FeTM4PyP 5+ ) was encapsulated between the layers of
MoS.~.
2. Experimental
To prepare the suspension of single layers of MoS:, pow-
dered 2H-MoS2 (~ 100 rag, Aldrich Chemical Co.) was
dried under vacuum (0.1 Torr) for 2 h and then flushed
several times with dry argon. LiBu" (5 ml, 2.4 mol 1- i solu-
tion in hexane, Aldrich) and hexane (5 ml) were then added.
The system was allowed to react under argon at 20°(2 for 5
days, according to Eq. (I) ix-- I ) [ 13,14].
2H-MoS,_ + xLiBu ~~x/2n-CsHxs + LidMo~ ( I )
After 5 days, tim ternary compound (Li)JloS,., ~ 20 rag)
was mixed with distilled water (50 ml) and sonicated for 2
h (4 × 30 min). This procedure yieldeda colloidal suspension
of single layers of MoS, (Eq. (2)).
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