DOI: 10.1007/s10967-008-7293-5 Journal of Radioanalytical and Nuclear Chemistry, Vol. 279, No.2 (2009) 611–617
0236–5731/USD 20.00 Akadémiai Kiadó, Budapest
© 2008 Akadémiai Kiadó, Budapest Springer, Dordrecht
Instrumental neutron activation analysis of water hyacinth
as a bioindicator along the Nile river, Egypt
Ashraf Aly Mohamed,
1
* H. A. Amer,
1
S. Shawky,
2
M. El-Tahawy,
1
A. T. Kandil
3
1
National Centre for Nuclear Safety and Radiation Control, Atomic Energy Authority, 3 Ahmed El-Zomor St.,
P.O. Box 7551, Nasr City, 11762 Cairo, Egypt
2
International Atomic Energy Agency, Wagramerstr. 5, P.O. Box 100, W-1400, Vienna, Austria
3
Helwan University, Faculty of Science, Chemistry Department, Ain Helwan, Cairo, Egypt
(Received June 16, 2008)
Water hyacinth (Eichhornia crassipes) is known to accumulate elements from rivers and a good tool for water monitoring. To test the usefulness of
such an aquatic plant as a bioindicator, we have determined the levels of Na, Ca, Cr, Fe, Co, Zn, As, Rb, Zr, Sb, Cs, La, Ce, Nd, Sm, Eu, Tb, Yb,
Hf, Ta, Th, and U in water hyacinth around industrial facilities and along the studied area by instrumental neutron activation analysis. The
concentrations of Cr, Mn, Fe, Co, Ni, Cu, Zn, Mo, Cd, and Pb were determined in upstream river water and effluent factories. Contamination
factor, and pollution load index was calculated. The results show that higher concentrations as well as bioaccumulation factors of these elements
were observed in water hyacinth samples around the industrial facilities. On the other hand a decrease in calcium concentration was observed as a
result of the thermal pollution of Nile river water. The pollution load index for the studied area was estimated to be 4.2.
Introduction
Environmental pollution has become a global
concern. One of the major areas of concern in Egypt is
the pollution of Nile river water by discharge from
industrial facilities. Huge quantities of industrial
effluents are discharged into the river. For example, the
cement factory, located at Tura area, Cairo discharges
6.9 million cubic meters per year, that contain about
400 kg from both Zn and Pb, as well as, about of 200 kg
Cu/year.
1
The excess of contaminants entering the
aquatic environment change the balanced bioavailability
and may enhance the toxicity to biological systems.
Biotransformation by bacteria in the water–sediment
interface can strongly influence elemental toxicity
throughout the remaining food chain. For example, Hg,
As, Sn, and Pb undergo biomethylation in the water–
sediment interface, resulting in the production of more
toxic species.
2
Thus environmental monitoring around
the discharge points of the industrial facilities is
necessary.
Using biological indicators such as plants for
monitoring both air and water pollution has been well
established. Alga is a sensitive indicator of metal
contamination in the aquatic environment.
3
Mosses have
been used extensively to monitor atmospheric deposition
of heavy metals and other trace constituents,
4
where
chemical analyses of these bioindicators are much easier
due to higher concentrations and strongly reduced
contamination problem,
5
especially when using non
destructive analysis technique such as instrumental
neutron activation analysis (INAA).
* E-mail: ashrafaly2001@yahoo.com
It was reported that water hyacinth successfully
absorbs and accumulates toxic elements from aqueous
solutions.
6–11
It was also used as a scavenger of heavy
metal pollutants in the Lake Chivero and its associated
rivers in Zimbabwe.
12
The absorption mechanisms of
these elements occur via the root system in substrate
water that was contaminated and via the leaves that were
exposed to atmospheric deposition.
11
ISMAIL et al.
1
determined Zn, Cu, and Pb in water hyacinth samples
collected from selected sites and water bodies around
greater Cairo. Results indicated that accumulation of the
element in question is due to its loading inputs in the
water body and water hyacinth is a good bioindicator
candidate for river water monitoring.
1
ASHRAF ALY et
al.
13
have concluded that water hyacinth is a good
bioindicator and bioaccumulator for uranium in Nile
river water and environmental impact of industrial
facilities were successfully monitored.
13
In this work we studied the usefulness of water
hyacinth as a bioindicator for environmental monitoring
especially around factories discharging their liquid
effluents into the Nile river. Water hyacinth, upstream
water and water discharge effluents at the same site were
collected from El-Saf city (south of Cairo) up to Rosetta
(Rachid Branch) to estimate the relative accumulation in
question due to its loading inputs in the water body.
INAA was used to determine the concentration of Na,
Ca, Sc, Cr, Fe, Co, Zn, As, Rb, Zr, Sb, Cs, La, Ce, Nd,
Sm, Eu, Tb, Yb, Hf, Ta, Th, and U in water hyacinth.
Concentrations of Cr, Mn, Fe, Co, Ni, Cu, Zn, Mo, Cd,
and Pb in upstream water and discharge effluents of
factories were determined by inductively coupled
plasma-atomic emission spectroscopy (ICP-AES).