Central European Journal of Chemistry
Dispersive liquid-liquid microextraction and
liquid chromatographic determination
of pentachlorophenol in water
* E-mail: kh.farhadi@urmia.ac.ir
Received 28 August 2008; Accepted 21 November 2008
Abstract: A simple and sensitive dispersive liquid-liquid microextraction method for extraction and preconcentration of pentachlorophenol
(PCP) in water samples is presented. After adjusting the sample pH to 3, extraction was performed in the presence of 1% W/V
sodium chloride by injecting 1 mL acetone as disperser solvent containing 15 µL tetrachloroethylene as extraction solvent.
The proposed DLLME method was followed by HPLC-DAD for determination of PCP. It has good linearity (0.994) with wide linear
dynamic range (0.1-1000 µg L
-1
) and low detection limit (0.03 µg L
-1
), which makes it suitable for determination of PCP in water samples.
© Versita Warsaw and Springer-Verlag Berlin Heidelberg.
Keywords: Dispersive liquid-liquid microextraction • Herbicide • Pentachlorophenol • Water sample • High performance liquid chromatography
1
Department of Chemistry, Faculty of Science,
Urmia University,
Urmia, Iran
2
Department of Analytical Chemistry, Faculty of Chemistry,
University of Tabriz,
Tabriz, Iran
3
Research Department of Chromatography,
Iranian Academic Center for Education, Culture & Research (ACECR),
Urmia, Iran
Khalil Farhadi
1*
, Mir A. Farajzadeh
2
, Amir A. Matin
1,3
, Paria Hashemi
1,3
Research Article
1. Introduction
Pentachlorophenol (PCP) has been used for over ifty
years as a herbicide in agriculture and an effective
preservative in wood industry [1]. PCP is classiied as
the 31st hazardous material in the list of environmental
protection agency (EPA) and also it is classiied
as a highly dangerous material by the world health
organization (WHO) [2,3]. PCP is extremely toxic when
ingested by humans; the probable oral lethal dose is 50 to
500 mg kg
-1
for a 70 kg person. Acute inhalation exposure
to pentachlorophenol in humans may result in death from
effects on the circulatory system and accompanying
heart failure. Tests involving acute exposure of animals,
such as the LC50 and LD50 tests in rats and mice,
have shown pentachlorophenol to have high toxicity
from inhalation exposure and extreme toxicity from oral
exposure.The maximum contamination level (MCL) for
PCP in drinking water is regulated at 1 ppb by EPA and
0.5 ppb by European Union [4] and it has various short
and long term harmful effects on human health.
Short term hazards include central nervous system
damage while long term hazards include cancer and
damage to the liver, kidneys and reproductive system [2].
It can get accumulated in the food chain due to its lipophilicity
and contaminates water and soil [5]. So in order to manage
environmental pollution and increase the drinking water
quality, there is a vital need to develop more sensitive
methods for PCP determination. Various analytical methods
such as spectrophotometric [6], liquid chromatographic
[7-9], gas chromatographic [10] and electrochemical
methods [11] have been developed for this purpose.
Despite technological advances in instrumentation
of chemical analysis, the resultant sensitivities are
Cent. Eur. J. Chem. • 7(3) • 2009 • 369-374
DOI: 10.2478/s11532-009-0013-3
369
Unauthenticated
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