ORIGINAL PAPER
Biodegradation of cyanide and evaluation of kinetic models
by immobilized cells of Serratia marcescens strain AQ07
K. I. Karamba
1,2
· S. A. Ahmad
1
· A. Zulkharnain
3
· N. A. Yasid
1
·
A. Khalid
4
· M. Y. Shukor
1
Received: 12 July 2016 / Revised: 10 January 2017 / Accepted: 15 February 2017
© Islamic Azad University (IAU) 2017
Abstract Immobilized form of Serratia marcescens strain
AQ07 was experimented for cyanide biodegradation.
Cyanide degradation (200 ppm) was achieved after 24-h
incubation. Three parameters were optimized which
included gellan gum concentration, beads size, and number
of beads. In accordance with one-factor-at-a-time method,
cyanide removal was optimum at 0.6% w/v gellan gum gel,
0.3-cm-diameter beads, and 50 beads number. It was able
to withstand cyanide toxicity of 800 ppm, which makes it
very suitable candidate in cyanide remediation. Beads
reusability indicates one-cycle ability. The first cycle
removed 96.3%, while the second removed 78.5%. Effects
of heavy metals at 1.0 ppm demonstrated that mercury has
a considerable effect on bacteria, inhibiting degradation to
61.6%, while other heavy metals have less effect, removing
97–98%. Maximum specific degradation rate of 0.9997 h
-1
was observed at 200 ppm cyanide concentration. Gellan
gum was used as the encapsulation matrix. ɤ-picoline-
barbituric acid spectrophotometric analytical method was
used to optimize the condition in buffer medium integrated
with potassium cyanide via one-factor-at-a-time and
response surface method. The range of cyanide concen-
trations used in this research, specific biodegradation rate
was obtained to model the substrate inhibition kinetics.
This rate fits to the kinetic models of Teisser, Aiba and
Yano, which are utilized to elucidate substrate inhibition
on degradation. One-factor-at-a-time approach parameters
were adopted because it removes more cyanide compared
to response surface methodology modules. The predicted
biokinetic constant from this model suggests suitability of
the bacteria for use in cyanide treatment of industrial waste
effluents.
Keywords Gellan gum · Immobilized · Kinetic models ·
Substrate inhibition
Introduction
Huge quantities of cyanide are used in industrial activities all
over the world. This includes electroplating, gold mining,
metal plating, coal gasification, pharmaceuticals, ore leach-
ing, plastics, aluminum electrolysis, and synthetic fiber
(Kjeldsen 1999; Yanase et al. 2000). Cyanide is considered
as one of the most toxic chemicals in the world. In living
organisms, it deactivates respiratory function of a living cell
by firmly binding to the terminal oxidase (Chena and Liu
1999; Yanase et al. 2000). In order to protect the environ-
ment, all cyanide-polluted waters need to be treated before
being discharged to the environment (Chen et al. 2008).
Several conventional treatment methods that are utilized in
Editorial responsibility: H.K. Pant.
& S. A. Ahmad
aqlima@upm.edu.my
1
Department of Biochemistry, Faculty of Biotechnology and
Bio-molecular Sciences, Universiti Putra Malaysia (UPM),
43400 Serdang, Selangor, Malaysia
2
Department of Microbiology, Faculty of Science, Bauchi
State University, Gadau Main Campus, Gadau, Bauchi State,
Nigeria
3
Department of Molecular Biology, Faculty of Resource
Science and Technology, Universiti Malaysia Sarawak,
Kota Samarahan, Malaysia
4
Faculty of Health Sciences, Universiti Kebangsaan Malaysia,
Jalan Raja Muda Abdul Aziz, 50300 Kuala Lumpur,
Malaysia
123
Int. J. Environ. Sci. Technol.
DOI 10.1007/s13762-017-1287-1