1. Introduction
In recent years, considerable research effort has
been devoted to the use of polymeric biodegradable
materials in plastics applications, such as packaging,
to reduce the environmental impact related to the
accumulation of plastics waste from the day-to-day
applications of plastic materials based on traditional
polymers, such as polyethylene terephthalate (PET),
polyethylene (PE), etc. [1, 2]. One of the promising
polymers used in these applications was the poly-
lactic acid (PLA), which was an aliphatic polyester
derived from lactic acid (2-hydroxypropionic acid)
[3].
First, PLA with a low-molecular weight was synthe-
sized by Carothers in 1932 [4, 5]. Further work by
DuPont resulted in a higher-molecular weight prod-
uct patented in 1954 [6]. Accordingly, two methods
were used to produce the basic block of PLA, lactic
acid (LA): the chemical synthesis was based on
petrochemical feedstock and carbohydrate fermen-
tation (Figure 1). Although the former was more
familiar to chemists, the fermentation of natural mate-
rials containing carbohydrates, such as rice, corn,
etc., was the main method used to produce LA
(>90%). Datta and Henry [7] examined the synthe-
sis and purification technologies of LA that were
found in two enantiomers, L- and D-lactic acid. The
results reported in that work showed that a 50/50
optically inactive mixture of L and D could be pro-
duced via a chemical route. In contrast, fermenta-
tion-derived lactic acid existed almost exclusively
as L-lactic acid. The ability to produce the L-isomer
in high purity possessed important ramifications in
chemistry and the ultimate process/property rela-
tionships achievable in the polymers produced from
lactic acid.
435
Properties and medical applications of polylactic acid:
A review
K. Hamad
1
, M. Kaseem
1
, H.W. Yang
1
, F. Deri
2
, Y. G. Ko
1*
1
Plasticity Control & Mechanical Modeling Laboratory, School of Materials Science & Engineering, Yeungnam
University, Gyeongsan 712–749, South Korea
2
Laboratory of Materials Rheology, Department of Chemistry, University of Damascus, Damascus, Syria
Abstract. Polylactic acid (PLA), one of the well-known biodegradable polyesters, has been studied extensively for tissue
engineering and drug delivery systems, and it was also used widely in human medicine. A new method to synthesize PLA
(ring-opening polymerization), which allowed the economical production of a high molecular weight PLA polymer, broad-
ened its applications, and this processing would be a potential substitute for petroleum-based products. This review
described the principles of the polymerization reactions of PLA and, then, outlined the various materials properties affect-
ing the performance of PLA polymer, such as rheological, mechanical, thermal, and barrier properties as well as the pro-
cessing technologies which were used to fabricate products based on PLA. In addition, the biodegradation processes of
products which were shaped from PLA were discussed and reviewed. The potential applications of PLA in the medical
fields, such as tissue engineering, wound management, drugs delivery, and orthopedic devices, were also highlighted.
Keywords: biodegradable polymers, polylactic acid, properties, medical applications
eXPRESS Polymer Letters V
Available online at www.expresspolymlett.com
*
Corresponding author, e-mail: younggun@ynu.ac.kr
© BME-PT