220 | wileyonlinelibrary.com/journal/cbdd Chem Biol Drug Des. 2018;91:220–14. © 2017 John Wiley & Sons A/S.
Received: 23 November 2016
|
Revised: 21 March 2017
|
Accepted: 8 July 2017
DOI: 10.1111/cbdd.13073
RESEARCH ARTICLE
Novel menadione hybrids: Synthesis, anticancer activity, and
cell-based studies
Chakka Vara Prasad
1
|
Vadithe Lakshma Nayak
2
|
Sistla Ramakrishna
2
|
Uppuluri Venkata Mallavadhani
1
1
Natural Products Chemistry
Division, CSIR-Indian Institute of Chemical
Technology, Hyderabad, India
2
Department of Medicinal Chemistry and
Pharmacology, CSIR-Indian Institute of
Chemical Technology, Hyderabad, India
Correspondence
Uppuluri Venkata Mallavadhani, Natural
Products Chemistry Division, CSIR-
Indian Institute of Chemical Technology,
Hyderabad, India.
Email: uvmavadani@yahoo.com
Funding information
Fellowship
A series of novel menadione-based triazole hybrids were designed and synthesized
by employing copper-catalyzed azide-alkyne cycloaddition (CuAAC). All the syn-
thesized hybrids were characterized by their spectral data (
1
H NMR,
13
C NMR, IR,
and HRMS). The synthesized compounds were evaluated for their anticancer activity
against five selected cancer cell lines including lung (A549), prostate (DU-145), cer-
vical (Hela), breast (MCF-7), and mouse melanoma (B-16) using MTT assay. The
screening results showed that majority of the synthesized compounds displayed sig-
nificant anticancer activity. Among the tested compounds, the triazoles 5 and 6 ex-
hibited potent activity against all cell lines. In particular, compound 6 showed higher
potency than the standard tamoxifen and parent menadione against MCF-7 cell line.
Flow cytometric analysis revealed that compound 6 arrested cell cycle at G0/G1
phase and induced apoptotic cell death which was further confirmed by Hoechst
staining, measurement of mitochondrial membrane potential (ΔΨm) and Annexin-
V-FITC assay. Thus, compound 6 can be considered as lead molecule for further
development as potent anticancer therapeutic agent.
KEYWORDS
1,2,3-triazole, 1,4-naphthoquinone, apoptosis, cell cycle arrest, cytotoxicity, menadione
1
|
INTRODUCTION
Quinones are widely distributed in nature as secondary me-
tabolites. Both natural quinones and their synthetic analogues
possess broad spectrum of biological activities, including
antifungal, antibacterial, antimalarial, antiviral, and antican-
cer activity.
[1–3]
Moreover, the quinone scaffold is present
in many clinically useful cancer drugs such as daunorubi-
cin, doxorubicin, saintopin, mitomycin, and mitoxantrone
(Figure 1). The most important chemical class in the qui-
none family is the 1,4-naphthoquinones. Recently, naturally
occurring 1,4-naphthoquinones such as menadione (vitamin
K3), juglone, and plumbagin have grabbed attention for their
significant anticancer activity against various cancer cell
lines as well as in vivo in animal models.
[4–6]
Particularly,
menadione has been reported to exhibit in vitro anticancer
activity against mammary, breast, hepatic, blood, bladder,
and oral cancer cell lines.
[7,8]
Menadione was effective even
against multidrug-resistant leukemia cell lines and parental
leukemia cell lines.
[9,10]
The main mechanism of the cyto-
toxicity of menadione in cancer cells involves the oxidative
stress via redox cycling of quinone to produce reactive ox-
ygen species (ROS), which leads to DNA damage and cell
death.
[11]
A phase I clinical study showed that menadione is
reasonably well tolerated, and menadione showed synergistic
cytotoxicity effect with other anticancer drugs such as 5-FU,
bleomycin, mitomycin C, and vitamin C.
[12]
Due to its re-
markable bioactivities, much more effort has been devoted in
synthesizing novel analogues of menadione with newer and
enhanced cytotoxic activities.
The triazole ring system is a very well-recognized phar-
macophore. This five-membered heterocycle is a prominent