IJSRSET1841310 | Received : 11 Feb 2018 | Accepted : 21 Feb 2018 | January-February-2018 [(4) 1 : 1396-1400 ]
© 2018 IJSRSET | Volume 4 | Issue 1 | Print ISSN: 2395-1990 | Online ISSN : 2394-4099
Themed Section : Engineering and Technology
1396
Naked Eye Detection of Thiols by using Pyrene based
Chemosensor in Aqueous Medium
Milind S. Thakare
1
*, Pravin M. Yeole
2
1
Synthetic Organic Research Lab, Department of Chemistry, Pratap College, Amalner, Maharashtra, India
2
PG Research Lab, Department of Chemistry, R. L. College, Parola, Maharashtra, India
ABSTRACT
Thiols are well known biological species plays a major physiological role. Sensitive and quantitative sensing
thiols is therefore of great significance to public health investigation A new Pyrene based turn-on fluorescent
probe based on the Anchoring and Unanchoring strategy for the selective detection of thiol was synthesized. The
pyrene potrntially used as the fluorophore and an DNBS group was combined as both a fluorescence quencher
and a recognition unit .which can react with thiol and releases the hydroxypyrene which has strong
fluorescence, The fluorogenic reaction is selectivel y initiated by the presence of thiols. The results indicate high
application potential in analytical chemistry and diagnostics.
Keywords : Thiols, Anchoring- Unanchoring, hydroxypyrene, DNBS, CTAB, Chemosensor.
I. INTRODUCTION
In last few decades there has been specific attention
on the chemosensing of mercaptans, as they play a
key role in extensive array of physiological processes
and biological functions
1-5
,biothiols such as
cysteine ,homocysteine, and glutathione are a
component of many amino acids and peptides,
Preservation of appropriate concentrations of these
low molecular-weight thiols is necessary for
numerous cellular functions, conversely, the
abnormal levels of thiols can give rise to various
health complications. For instance, the inadequacy of
Cys contribute to slowed growth in children, hair
depigmentation, edema, lethargy, liver damage, loss
of muscle and fat, skin lesions, and weakness,an
elevated level of Hcy in human plasma is a risk factor
for Alzheimer’s, cardiovascular diseases, neural tube
defect, and coronary heart disease
6-14
. Therefore, a
rapid, sensitive, and selective detection of thiols in
biological samples is of significance.
Typical instrumental detection methods for biothiols
include liquid chromatography, capillary
electrophoresis, voltammetry and flow injection
15-20
.
However, those techniques require relatively complex
sample preparation protocols and sophisticated
instrumentation. Among various methods for
detection of biothiols, the fluorescence method
21-41
based on fluorescence probe is expedient due to its
desirable features such as high sensitivity, simplicity,
and potential for in vivo imaging . Noteworthy efforts
have been devoted to construction of fluorescent
probes for biothiols . Many fluorescent probes,
involved in different detecting mechanisms, have
been developed for thiols detecting, such as Michael
addition reaction
42
, cyclization reaction based on
aminothiols and aldehyde , cleavage reaction induced
by thiols ,and ligand displacement of metal complexes
by thiols.
21-41
The thiol mediated nucleophilic displacement
strategy
43
provides a superior performance of
chemosensors for recognition of thiols. However, it is