IJSRSET184433 | Received : 01 March | Accepted : 12 March 2018 | March-April-2018 [(4) 4 : 171-177 ]
© 2018 IJSRSET | Volume 4 | Issue 4 | Print ISSN: 2395-1990 | Online ISSN : 2394-4099
Themed Section : Engineering and Technology
171
Photoluminescence, Photoconductivity, Thermal,
Microhardness and Dielectric Properties of Silver Nitrate
Doped Potassium Zinc Phosphate Hexahydrate Single Crystal
R. Azhagu Raj
*1
, Ambrose Rajkumar Mariadass
2
, D. Krishnamoorthy
3
, A. Prakasam
3
,
Prem Anand Devarajan*
2
1
Department of Zoology, St. Xavier's College (Autonomous), Palayamkottai, Tamil Nadu, India
2
Department of Physics, St. Xavier's College (Autonomous), Palayamkottai, Tamil Nadu, India.
3
Department of Physics, Thiruvalluvar Govt. Arts College, Rasipuram, Tamil Nadu, India
ABSTRACT
Silver nitrate doped potassium zinc phosphate hexahydrate NLO single crystal was grown using conventional
solution growth technique. The as grown single crystal was subjected to single crystal X-ray diffraction and it
was revealed that crystal belongs to monoclinic system. Photoluminescence spectra was observed at 415 nm
and 545 nm due to the π* - n and π- π* transitions. Photoconductivity was measured to understand the internal
processes in crystals. The negative conductivity of the as grown crystal may be due to the reduction in number
of charge carries in the presences of radiation. Thermal properties of silver nitrate doped potassium zinc
phosphate hexahydrate were studied and it was found that the melting point of as grown is 123
0
C.
Microhardness of silver nitrate doped potassium zinc phosphate hexahydrate was also studied and concluded
that it belongs to soft material. Electrical property of as grown crystal was also carried out.
Keywords : Potassium zinc phosphate hexahydrate, Photoluminescence, Dielectric, monoclinic and
microhardness
I. INTRODUCTION
New materials exhibiting non linear optical (NLO)
effects have been explored with view to develop opto-
electrical devices for example optical modulator and
frequency doubling devices [1]. Hence the search for
efficient non linear optical (NLO) crystals is in fact
that search for the polar crystals in which the
macroscopic properties reflect the internal
asymmetric molecular relationship. Such a crystal
may have an external morphology with hemi hedral
faces that have different chemical reactivity and
physical properties, such as third order NLO activity
in addition to pyro electric, pizzo electric and ferro
electric effects [2]-[3]. The unique property of perfect
single crystals was employed in the development of
device fabrications in semiconductors, optics,
photonics, nonlinear optics, light-emitting diodes,
faster processors, high- resolution detectors,
ferroelectric and piezoelectric applications[4-6]. The
numerous applications of the nonlinear optical (NLO)
crystals in the vast field of science and technology
made the process of search of the new NLO crystals
and improvements in the properties of the known
crystals a never stopping process. Purely inorganic
NLO materials typically have excellent mechanical
and thermal properties but often posses relatively
modest optical nonlinearities due to their lack of
extended π- electrons delocalization. Furthermore
inorganic crystals grown from high temperature melts
typically have lower damage thresholds and more
optical inhomogeneties throughout their bulk due to