IJSRST1841138 | Received : 15 Jan 2018 | Accepted : 02 Feb 2018 | January-February-2018 [ (4) 2: 587-582]
© 2018 IJSRST | Volume 4 | Issue 2 | Print ISSN: 2395-6011 | Online ISSN: 2395-602X
Themed Section: Science and Technology
587
Synthesis, Characterization and Evaluation of Biological Properties of
Transition Metal Chelates with Schiff base Ligands Derived from
Glutaraldehyde with L-Leucine
S. Ajith Sinthuja, Y. Christabel Shaji , G. Leema Rose
Department of Chemistry, Holy Cross College (Autonomous), Nagercoil, Tamil Nadu, India
ABSTRACT
A nitrogen-oxygen Schiff base HL derived from Glutaraldehyde and L-Leucine has been reacted with different
divalent metal ions in 2:1 molar ratio, producing neutral complexes . All compounds were characterized using
physico-chemical and spectroscopic methods namely elemental analysis, melting point, magnetic moment
measurement, conductivity measurement, UV-Vis, IR,
1
HNMR spectroscopy and XRD measurements. They
were further analysed by thermal technique (TGA/DTA) to gain better insight about the thermal stability and
kinetic properties of the complexes. The IR data demonstrated the tetradentate binding of Schiff base ligand.
The molar conductivity values were relatively low , showing their nonelectrolytic nature. Room temperature
magnetic susceptibility measurements revealed that the nature of Ni(II) and Cu(II) complexes were
paramagnetic. The in vitro antimicrobial activities of all the compounds were screened against different
microbial species by Disc Diffusion method and showed better activity compared to parent drug and control
drug.
Keywords: Schiff base, Metal complexes, IR, XRD, Antimicrobial activity
I. INTRODUCTION
Transition metal complexes derived from Schiff bases
have occupied a central role in the development of
coordination chemistry. Schiff base can accommodate
different metal centers involving various coordination
modes thereby allowing successful synthesis of homo
and hetero metallic complexes with varied
stereochemistry .This feature is employed for
modeling active sites in biological systems. A large
number of Schiff bases and their complexes have been
investigated for their interesting and important
properties, such as their ability to reversibly bind
oxygen, their catalytic activity in the hydrogenation
of olefins, their photochromic properties and their
complexing ability towards some toxic metals. Many
biologically important Schiff bases have been reported
in the literature possessing, antimicrobial,
antibacterial, antifungal, anti-inflammatory, anti
convulsant, antitumor and anti- HIV activities
(1-4)
. In
vivo studies have indicated that some biologically
active compounds may become more carcinostatic and
bacteriostatic upon chelation
(5)
. Several reviews
showed that the metallo-organic chemistry of such
compounds greatly influence their biological action
highlighting the catalytic function metal in many
biological processes
(6-8)
.
Therefore, considering the above facts and continuing
our interest in this field, the present work reports a
study on the synthesis, characterization and
antimicrobial properties of Ni and Cu complexes with
the Schiff base derived from Glutaraldehyde and L-
Leucine (HL).
II. EXPERIMENTAL
Materials and Physical Measurements:
All the glassware used for the preparation were
cleaned with chromic mixture ,distilled water and
then dried in Oven at 110
o
C. All the chemicals such as
Glutaraldehyde, L- Leucine, Cupric nitrate and Nickel