IJSRST1841211 | Received : 25 Jan 2018 | Accepted : 08 Feb 2018 | January-February-2018 [ (4) 2: 869-876]
© 2018 IJSRST | Volume 4 | Issue 2 | Print ISSN: 2395-6011 | Online ISSN: 2395-602X
Themed Section: Science and Technology
869
Preparation, Photoluminescent Behaviour, Antimicrobial and
Antioxidant Properties of New Orange Light Emitting Sm(III)
Complex, Sm(CHME)
3
.Dmphen
P. Nandal
1
, R. Kumar
2
, Sheetal
1
, S. P. Khatkar
1
, V. B. Taxak
1
*
1
Department of Chemistry, Maharshi Dayanand University, Rohtak, Haryana, India
2
Department of Chemistry, UIET, Maharshi Dayanand University, Rohtak, Haryana , India
*
Corresponding Author: E-mail address: v_taxak@yahoomail.com
ABSTRACT
The photoluminescent properties of lanthanide complexes with organic ligand have been the subject of great
interest as these functional complexes have potential applications in various fields from quantum cutting
materials to photonic devices [1-13]. Most of these applications are based on the efficient emission of
lanthanide complexes in the UV region to IR regions. However, the lanthanide ions have very low absorption
coefficient which prevents direct excitation due to Laporte-forbidden 4f-4f transitions. To overcome this
disadvantage and obtain intense lanthanide luminescence, there are two specific ways to sensitize lanthanide
emission. Firstly, the use of metal ion in the heteromettalic system where energy can be transferred from the
metal ion to lanthanide ion which results in enhanced luminescence of lanthanide ion. Secondly, to choose a
suitable organic chromophore moiety which excite and transfers the energy to the lanthanide ion through
antenna affects. For the second option numerous organic ligands such β-hydroxyketone, β-diketone, carboxylic
acids and various heterocyclic derivatives have been introduced to develop and designed new luminescent
lanthanide-based materials [14-20].
Keywords : Laporte-Forbidden, Photoluminescent, Antimicrobial, Antioxidant, Sm(CHME)3.Dmphen, UV
Region, IR Regions, Organic Chromophore Moiety, Β-Hydroxyketone, Β-Diketone, Carboxylic Acids, CHME,
OLEDs
I. INTRODUCTION
The β-hydroxyketones and its derivatives serve as
excellent antennas or sensitizers, absorbing the
excitation light and transferring the energy to the
trivalent lanthanide ions [21-24]. The choice of β-
hydroxyketone ligand is based on its strong ability to
coordinate lanthanide ion which can have many
practical usage. To the best of the author knowledge,
Eu
3+
and Tb
3+
ions are of particular interest but
investigations on Sm
3+
complexes containing β-
hydroxyketone ligand are still rare. This present work
deals with the synthesis of a new Sm(III) complex
employing β-hydroxyketone ligand 2-(4-
chlorophenyl)-1-(2-hydroxy-4- ethoxyphenyl)ethan-
1-one (CHME) as main ligand and 5,6-dimethyl-1,10-
phenanthroline as ancillary ligands. The investigation
of photoluminescent properties has also done for
possible use in OLEDs as emitting materials. The
author also explicated in vitro antimicrobial activities
and antioxidant activities of ligand and its
corresponding Sm(III) complex employing tube
dilution method and DPPH method respectively in
detail.