IJSRST1184893 | Received : 07 June 2018 | Accepted : 18 June 2018 | May-June-2018 [ 4 (8) : 517-525]
© 2018 IJSRST | Volume 4 | Issue 8 | Print ISSN: 2395-6011 | Online ISSN: 2395-602X
Themed Section: Science and Technology
517
Removal of Reactive Scarlet Dye and COD Using Cylindrical Iron
Rod Anodes In A Semi-Continuous Reactor
Ersin Aytac
1*
, Umran Tezcan Un
2
1
Department of Environmental Engineering, Zonguldak Bülent Ecevit University, Zonguldak, Turkey
2
Department of Environmental Engineering, Eskisehir Technical University, Eskişehir, Turkey
ABSTRACT
The cylindrical iron electrochemical reactor for electrocoagulation (EC) of reactive scarlet dye was studied. In
the study, 0.5 L synthetic wastewaters with a dye concentration of 200 mg/L and chemical oxygen demand of
620 mg/L (COD) prepared in laboratuary treated for 90 minutes of EC. The effects of operational parameters
such as current density (10 - 30 mA/cm2), initial pH (5 - 9), flow rate (100 - 400 mL/min) and the supporting
electrolyte concentration (0.05 - 0.2 M Na2SO4) were investigated. For each operation parameter, dye stuff
concentration and chemical oxygen demand has been measured for removal efficiencies after treatment
duration. To estimate the operating cost, the electrical energy consumption was calculated. It has been observed
that current density has positive effect on removal efficiencies. Moreover adequate dye stuff removals has been
achieved in short process time and low current efficiencies. When effect of the initial pH value of the
wastewater was examined, it was observed that the optimum pH value was 7.1. When investigating the
influence of flow rate it was found that higher flow rates has ngative effect by breaking up the aggregates. The
lowest electrical energy consumptions has been established in 0.2 M Na2SO4 concentration for the effect of
supporting electrolyte concentration. Effluent COD concentration of 22 mg/L with a removal efficiency of
96.5% and effluent dye concentration of 1.08 mg/L with a removal efficiency of 99.46% was obtained with an
electrical energy consumption of 4.28x10-4 kWh/mg CODremoved. Additionally, the sludge produced at
electrocoagulation was characterized and maghemite (Fe2O3) was found as most common species.
Keywords : COD Removal, Decolorization, Electrochemical Treatment, Iron Electrode, Reactive
I. INTRODUCTION
Increasing population and industrialization can affect
human life and the environment either positively or
negatively. Engineering science is able to formulate
the necessary precautions to ensure a sustainable
environment and natural life. In the last few decades,
new developments in treatment technologies have
been seen. Development in wastewater treatment is
essential for lessening the harmful effects of industrial
waste on the environment. Electrocoagulation (EC), in
conjunction with wastewater treatment processes, has
become prominent in recent years. EC is an electro-
chemical process in which electrically oxidized metals
have the ability to form coagulants by combining with
electrolyzed water, in situ. In fact, in EC, not only do
metal hydroxides form as coagulants, but other
mechanisms also occur. Floating and electro-chemical
reactions are amongst these treatment mechanisms.
Aluminum and iron electrodes are mostly used in EC
because of their cost of effectiveness, availability and
effectiveness in the formation of coagulants.
The ion charge of oxidized metal can be different
depending on the voltage applied. Reactions occurring
with iron electrodes are shown below [1];
Mechanism I