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Drug Delivery Letters, 2014, 4, 000-000 1
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Optimization and Formulation of Cinnarizine-Loaded Chitosan Micro-
spheres in Liquid Dosage Form for Pediatric Therapy
Reham Aman
*
, Mahasen Meshali and Galal Abdelghani
Department of Pharmaceutics, Faculty of Pharmacy, Mansoura University, Mansoura, 35516, Egypt
Abstract: Cinnarizine pediatric preparation is extemporaneously prepared from adult tablets or capsules that are unstable
in liquid dosage form. The aim of this work is to develop cinnarizine oral pediatric formulation with improved stability
and organoleptic properties as well as to achieve ease of administration. For this purpose, cinnarizine-loaded microspheres
of chitosan cross-linked with tripolyphosphate anion were prepared. A full 2
3
factorial design of experiment approach was
employed to evaluate the individual and the combined effect of the independent variables namely, concentration of each
of chitosan (X
A
), tripolyphosphate (X
B
), and that of cinnarizine (X
C
) on the different responses namely drug entrapment
efficiency, drug content, percentage yield and drug release rate for the prepared microspheres. Statistical analysis through
response-surface methodology as well as contour plots was assessed. The optimized microspheres (formula 4) showed
93.6±3.3 % percentage yield, 74.3±0.8 mg drug loading, 74.3±0.8 % encapsulation efficiency and 0.19 µm particle size.
Hence, it was subjected to stability study of cinnarizine in the dry microspheres immediately thereafter preparation
through transmission electron microscope, x-ray diffractometry, Fourier transform infrared spectroscopy and differential
scanning calorimetry. The microspheres were further dispensed in the prepared syrup and the suspension was subjected to
accelerated stability study, as mentioned in the International Conference on Harmonization (ICH) guidelines. Subse-
quently, oral bioavailability study of (formula 4) microspheres was conducted on rats and compared with aqueous suspen-
sion of the plain drug. Formula 4 complied successfully with ICH guidelines and experienced enhanced extent of
bioavailability with long mean residence time (MRT).
Keywords: Bioavailability, chitosan, cinnarizine, factorial design, microspheres, pediatric therapy.
INTRODUCTION
Cinnarizine (CIN) (1-benzhydryl 1-4-cinnamyl piperazine)
is a piperazine derivative that was firstly synthesized by
Dr. Paul A.J. Janssen in 1955 [1]. It is slightly soluble and
permeable and can be classified as class II (Biopharmaceuti-
cal Classification System) BCS [2]. Moreover, it is used in
vertigo, Meniere's disease, loss of memory and motion sick-
ness pharmacotherapy. The drug improves blood flow to the
labyrinth and brain stem and thus it is useful in cerebrovas-
cular and peripheral disorders [1].
The current commercially marketable dosage forms for
CIN are tablets and capsules for adults. Both of these dosage
forms exhibit low and erratic oral bioavailability. Several
intravenous dosage forms were investigated to overcome
these problems [3, 4]. However, the lack of commercially
available oral liquid dosage form for CIN makes it difficult
for using with children and infants as well. Hence, a pharma-
cist is often challenged to provide an extemporaneous oral
liquid formulation from a commercially available adult oral
solid dosage form by simply opening a capsule and the sub-
sequent addition of water or juice to overcome this problem
[5].
*Address correspondence to this author at the Department of Pharmaceutics,
Faculty of Pharmacy, Mansoura University, Mansoura, 35516 Egypt;
Tel: +050 2247496; E-mail: reham.aman@yahoo.com
Nevertheless, the dose adjustment to children's body
weight raised significant concern. In addition, organoleptic
drawbacks (e.g. bitterness) have an impact on patient com-
pliance and adherence [6]. The latest World Health Assem-
bly (WHA) stressed the importance of recognizing children's
right to access safe, effective, and proven medicines [7, 8].
Since no liquid formulation of CIN is available, an oral pedi-
atric dosage form is highly desirable.
Consequently, the aim of this work was to develop pedi-
atric oral liquid formulation of CIN enabling convenient
dose adjustment, ease of administration and improved or-
ganoleptic properties. A method of choice was to load the
drug in microspheres prepared from natural polymer and
subsequently suspend them in the prepared syrup. Micro-
spheres have shown advantages as drug carriers [9]. Recent
concepts of microspheres formulations for pediatric use were
applied [10, 11].
The polymer of choice should be insoluble in the pre-
pared syrup but dissolved in the gastro-intestinal tract. A
natural polymer suitable for this purpose is chitosan, (CS)
[9]. It is stable, biocompatible and bioadhesive [12, 13]. CS
microspheres were used to improve the bioavailability as
well as to enhance the uptake of hydrophilic substances
across epithelial membrane [14]. Optimized CIN-loaded CS
microspheres (CIN–CS) were prepared by adopting factorial
design 2
3
with three different independent variables at two
levels. Sodium tripolyphosphate (TPP) was the cross-linking