162 Int J Petrochem Res.
ISSN: 2638-1974
Volume 2 • Issue 2 • 1000128
International
Journal of Petrochemistry and Research
Research Article Open Access
Microwave assisted rice husk based activated carbon
for adsorption of methylene blue dye
Mohd Azmier Ahmad
1,3
*, Nor Irwin Basir
1
and Nasehir Khan EM Yahaya
2
1
School of Chemical Engineering, Engineering Campus, UniversitiSainsMalaysia, 14300 NibongTebal, Penang, Malaysia
2
National Hydraulic Research Institute of Malaysia, Lot 5733 Jalan Putra Permai, 43300 Seri Kembangan, Selangor, Malaysia
3
Solid Waste Management Cluster, Science & Engineering Research Centre, Engineering Campus, UniversitiSains Malaysia,
NibongTebal, Penang, Malaysia
Article Info
*Corresponding author:
Mohd Azmier Ahmad
School of Chemical Engineering
Engineering Campus, Universiti Sains
Malaysia
14300 Nibong Tebal
Penang, Malaysia
Tel: +604 5996459
Fax: +604 5996908
E-mail: chazmier@usm.my
Received: July 25, 2018
Accepted: July 31, 2018
Published: August 5, 2018
Citation: Ahmad MA, Basir NI, Yahaya NKEM.
Microwave assisted rice husk based activated
carbon for adsorption of methylene blue
dye Int J Petrochem Res. 2018; 2(2):
162-164.
doi: 10.18689/ijpr-1000128
Copyright: © 2018 The Author(s). This
work is licensed under a Creative Commons
Attribution 4.0 International License, which
permits unrestricted use, distribution, and
reproduction in any medium, provided the
original work is properly cited.
Published by Madridge Publishers
Abstract
Rice husk based activated carbon (RHAC) was prepared for the methylene blue (MB)
dye adsorption through physical activation process which involved microwave irradiation
and carbon dioxide gasification. The effect of initial dye concentration and contact time
were evaluated in a batch process. The MB adsorption onto RHAC was found to increase
from 16.18 to 137.15 mg/g as the MB concentrations increase from 25 to 300 mg/L. The
adsorption equilibrium data was best fitted into Freundlich isotherm model.
Keywords: Activated carbon, Adsorption, Methylene blue, Microwave heating, Rice husk
Introduction
The textile is one of the largest water consuming industries and releases large
amount of effluent. The textile effluent contains carcinogenic dye, toxic heavy metals,
phenolic compounds, softeners and other chemicals used in the dyeing process [1]. The
presences of even very low concentration of dye in the effluent are highly visible and
undesirable. Dye is very much associated with carcinogenic, mutagenic, allergenic and
toxic properties [2]. Dye is difficult to be decolorized and decomposed biologically.
Therefore, the dye wastewater needs to be properly treated before its release into the
environment [3]. Activated carbon (AC) adsorption is considered as one of the most
effective method for dye wastewater treatment [4]. In this study, rice husk was used to
produce AC using microwave heating and CO
2
gasification for MB dye removal from
aqueous solution.
Methodology
The rice husk was placed in tubular reactor and carbonized using vertical furnace at
temperature of 350°C for 30 minutes under the nitrogen flow of 150 ml/min. Then the
char produced was placed in a Pyrex glass reactor in the chamber of the microwave
oven. The microwave irradiation was carried at radiation time and radiation power of
4.28 minutes and microwave power of 440 watt under CO
2
flow of 150 ml/min.
For adsorption study, the 1 g/L of MB stock solution was prepared by dissolving 1 g
of MB dye powder (Sigma-Aldrich (M) Ltd) with 1 litre of deionized water. 0.2 g of the
RHAC was added to a series of Erlenmeyer flask filled with 0.2 L of MB dye solution with
different initial concentrations ranging from 25-300 mg/L. The solutions were kept in an
isothermal water bath shaker at temperature 30
o
C and shaker speed of 60 rpm. The
aqueous samples were then withdrawn at the equilibrium state of 24 hours. The MB
concentration was measured at 664nm by using UV-Vis spectrometer (Model Shimadzu
ISSN: 2638-1974