Optik 138 (2017) 372–376
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Optik
j o ur nal ho me pa ge: www.elsevier.de/ijleo
Short note
Dose dependence effect of thermoluminescence process in
TlInS
2
:Nd single crystals
Ahmed Kadari
a,∗
, Serdar Delice
b
, Nizami Mamed Gasanly
c,d
a
Department of Chemistry, Faculty of Sciences of the Matter, Ibn Khaldoun University of Tiaret, BP P 78 Zaaroura, Tiaret, Algeria
b
Department of Physics, Hitit University, 19030 C ¸ orum, Turkey
c
Department of Physics, Middle East Technical University, 06800 Ankara, Turkey
d
Virtual International Scientific Research Centre, Baku State University, 1148 Baku, Azerbaijan
a r t i c l e i n f o
Article history:
Received 12 December 2016
Accepted 15 March 2017
Keyword:
Thermoluminescence
Trap parameters
OTOR
Dose response
TlInS2:Nd
a b s t r a c t
In this paper, thermoluminescence (TL) properties of TlInS
2
:Nd single crystals were mod-
eled using an interactive model (one trap and one kind of recombination center). The
simulated work presented here was based on the experiment conducted by Delice et al.
The thermoluminescence glow curve of TlInS
2
:Nd single crystals has been characterized
by one main peak at 26 K, which confirm the presence of one active electron trap level in
the forbidden band of this material. The model used in this work is similar to other mod-
els cited previously in the literature. The calculated glow curve was in good agreement
with the experimental one. Our numerical results show also that the thermoluminescence
intensity increases with the increase of the dose rate (D). In the selected dose level range;
the thermoluminescence response is linear and no saturation can be observed.
© 2017 Elsevier GmbH. All rights reserved.
1. Introduction
Lately, ternary compounds of semiconductor materials have become a significant subject for researchers and studies
on them have gain considerable momentum. Their optical, structural and electrical capabilities [1–4] show that they carry
remarkable potential to be used in producing optoelectronic devices. Ternary TlInS
2
is a member of semiconducting mate-
rials consisted of III and VI elements in periodic table and it possesses layered structure. The ionic-covalent bonds occur
between the atoms whereas the weak van der Waals bonds are created between the sequential two-dimensional layers
that are perpendicular to the (001) direction. The space group of C
6
2h
characterizes the crystal symmetry of TlInS
2
, which has
monoclinic structure at room temperature [5,6]. Among ternary layered crystals, TlInS
2
was mostly preferred material by
researchers. The physical properties of TlInS
2
crystal were widely investigated and reported in literature [7–11].
Several experimental techniques and simulations under the light of the theoretical models were applied for different
materials in literature to characterize the trapping process of defects. TlInS
2
single crystals were studied by using the
thermally stimulated current (TSC), photoluminescence (PL) and thermoluminescence (TL) measurements. The TSC inves-
tigations achieved in 10–90 K [12] and 100–300 K [13] temperature regions revealed the existence of five trapping levels
centered at energies of 12, 14 meV [12] and 400, 570 and 650 meV [13], respectively. The PL spectra detected between 500
and 850 nm and in the temperature range 11.5–100 K established the existences of one donor level at 250 meV and one
acceptor level at 20 meV in the band gap [14]. Five trapping levels with thermal activation energies of 14, 19, 350, 420 and
∗
Corresponding author.
E-mail addresses: kadariahmed 14@yahoo.fr, ahmed.kadari27@gmail.com (A. Kadari).
http://dx.doi.org/10.1016/j.ijleo.2017.03.062
0030-4026/© 2017 Elsevier GmbH. All rights reserved.