International Journal of Aerospace Sciences 2016, 4(1): 9-13
DOI: 10.5923/j.aerospace.20160401.02
Performance of Epoxy and Nanodiamond Exfoliated
Montmorillonite Nanocomposite
Ayesha Kausar
Nanoscience and Technology Department, National Centre For Physics, Quaid-i-Azam University Campus, Islamabad, Pakistan
Abstract This report investigates the possibility of improving the mechanical properties of triglycidyl para-amino phenol
(TGAP) epoxy through dispersion of nanodiamond (ND) and montmorillonite-nanodiamond (MMT-ND) filler. The
montmorillonite was first intercalated with octadecylamine followed by nanodiamond intercalation to form MMT-ND. Both
the pristine nanodiamond as well as MMT-ND was employed as filler to form nanocomposite with triglycidyl para-amino
phenol. In this case, diethyltoluene diamine was used as hardener. It was found that the presence of nanofiller steadily
decreased the β-transition temperature of TGAP/ND and TGAP/MMT-ND systems. Atomic force micrographs have shown
fine particle dispersion in nanocomposite. The effect of filler concentration on mechanical properties of epoxy resins was also
analyzed. TGAP/ND 1-5 system showed increase in modulus from 1676 to 3074 MPa, while greater modulus increase was
seen for TGAP/MMT-ND 1-5 system in the range of 2388-3408 MPa. The balanced properties justified the application of
novel epoxy nanocomposites in aviation industry.
Keywords Epoxy, Montmorillonite, Nanodiamond, Intercalation, Modulus
1. Introduction
In aircraft and propulsion system, the main attention of
airplane designers was on the achievement of lightweight
materials [1]. Because of larger part to limited ability of
propulsion systems, absolute minimum weight was essential
for practical flight from 1903 to 1930. Subsequently, the
basic need for material choice in both aircraft and engines is
strength to weight ratio. While the concern remains to be first
order of significance, light weight is not only sufficient but
necessary. Recent criteria for design is very complex and
thus new design routes as well as increased constituents and
processing routes are required by winning products [2]. A
well-recognized family of thermosetting polymers is epoxy
resins. They have been extensively employed in numerous
industrial fields mainly high performance adhesives,
coatings and other engineering applications due to their
remarkable features. Moreover, the cured epoxy resin
possesses low impact strength, low fracture toughness, poor
resistance to crack initiation, and growth. Over the past
decade numerous investigations have been carried out to find
route for epoxy matrix toughening especially by the addition
of second phase mainly elastomeric or rigid constituents
[3-5]. Currently, it was found that the nanoclay fillers have
high modulus (170 GPa) and high aspect ratio (200-1000).
* Corresponding author:
asheesgreat@yahoo.com (Ayesha Kausar)
Published online at http://journal.sapub.org/aerospace
Copyright © 2016 Scientific & Academic Publishing. All Rights Reserved
Owing to their excellent properties they have developed a
new route for enhancement of mechanical potential such as
impact resistance and toughness of cured epoxy matrix [6].
Due to their low cost and ease of availability, clays have
fascinated remarkable interest. Additionally, the probability
of achievement of properties with nanoclay was achieved
with microscopic fillers. For aerospace applications and
automotive industries (in which composite material density
is required), low filler content is particularly needed [7].
Therefore, the low filler content is the demand of perfect
structure of polymer layered silicate nanocomposites. Thus,
clay act as conventional filler than that of exfoliated
nanocomposite. In order to restrict the cracks propagation
and increase the surface contact between clay and matrix,
uniform distribution of clay may occur in matrix. The
untreated nanoclay mainly montmorillonite (MMT) is
comprised of silicate layer stacks. Each of stack is about 1
nm in thickness and is hydrophilic naturally. The silicate
layer stacks are not appropriate for employment as filler in
most commonly utilized epoxy resin which is hydrophobic
[8]. Consequently, the montmorillonite clay is usually
altered organically by an ion exchange process in which the
cations are replaced by anions (as replacement of quaternary
ammonium ions with long alkyl chains). By this route the
spaces between clay layers increases which makes them
organophilic. The epoxy resin intercalation in the
preparation of epoxy/clay nanocomposites is strongly
facilitated by ion exchange method. In order to fulfill the
desired enhancement in mechanical features of these
composites, it is essential to further separate the clay layers