Applied Chemical Engineering (2018) Volume 1
doi: 10.24294/ace.v1i4.615
1
An overview to photo-catalytic degradation of dyes in waste water
Mohd. Hanief Najar
1
, Ishtiyaq Ahmed Najar
2
1
Department of Chemistry, Govt. College of Engineering and Technology Safapora, Ganderbal-191201, J&K India
2
Department of Environmental science, Govt. Degree College Ganderbal-191201, J&K India
ABSTRACT
Organic dyes used in textile and food industries are the important sources of environmental contaminations due to
their non-bio degradability and high toxicity to aquatic creatures and carcinogenic effects on humans. This demands
environmental remediation by the use of techniques which are environmentally benign. For this purpose, a general
overview of dye degradation by light in the presence of materials as photo-catalysts has been given. The mechanism of
action has also been described. Importantly, the materials involved in dye degradation usually involve nano-composites
of either conducting polymers or metal-oxidesor graphene based systems which are insoluble in aqueous solutions,
hence will be environmentally benign and can therefore be recovered after use.
Keywords: Nano-materials; Organic dyes; Photo-catalysis
1. Introduction and criteria for
materials to be best photo-catalysts
for dye degradation
The use of dyes in textile industries has become a
serious environmental issue because of the unacceptable
color of dye effluents, high chemical oxygen demand and
resistance to bio-degradation on account of having com-
plex aromatic structures. For this purpose, dyes in waste
water are either removed by adsorption or degraded by
photo-catalysis. In this area, semiconductor materials
have attracted much attention. Among semiconductors,
TiO
2
is considered a bench mark photo-catalyst for dye
degradation. This is because of having high efficiency,
low cost, chemical corrosion inertness, and long-term
stability against photo-corrosion and chemical corrosion.
Moreover, it is a photosensitive material, possesses high
photo-catalytic activity, is stable in aqueous systems and
has low environmental toxicity
[1]
.But the major short-
coming to the use of TiO
2
photo-catalysts lies in having
low quantum efficiency and the confined utilization of
sunlight. For a material to exhibit high photo-catalytic
activity, it must be porous and possess high surface to
volume ratio so as to lead increased adsorption of dye.
The high surface to volume ratio (surface area) can be
attained provided the material to be either highly porous
or nano-sized. This is the reason that benchmark
TiO
2
photo-catalyst has been found to be less efficient
than nano-sized TiO
2
.The material must exhibit slower
recombination rate of photo-generated electron-hole
pairs. This will help to cause facile degradation of dyes.
ZnO was found to have almost same band gap energy as
that of TiO
2
, hence it was anticipated to be a better an
alternative for TiO
2
photo-catalysts, but the fast recom-
bination rate of photo-generated charge carriers limits its
applicability. Reduction in the recombination rate can be
attained by forming hetero-junctions between different
components. This is indicative of making a composite
material. However, this would demand the proximal in-
terface contact. Moreover, materials with wider absorp-
tion range lead to enhanced efficiency in the degradation
of dyes. For such a factor, TiO
2
again has limited ap-
plicability as it absorbs only a small portion of UV light.
Thus to widen its absorption band spectrum, doping,
composite science and the formation of hetero-junctions
is essential. All the factors discussed above are comple-
mentary to one another. This we mean to say that a mate-
rial with high surface to volume ratio does not suffice
to be a good photo-catalyst unless other factors are more
or less favoring. This demands the balance in the proper-
ties of materials desirable for photo-catalysis
[2-5]
.
Copyright © 2018 Mohd. Hanief Najar et al.
doi: 10.24294/ace.v1i4.615
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