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Nuclear Engineering and Design
journal homepage: www.elsevier.com/locate/nucengdes
Experimental study of transient phenomena in the three-liquid oxidic-
metallic corium pool
V.I. Almjashev
a,
⁎
, V.S. Granovsky
a
, V.B. Khabensky
a
, S.Yu. Kotova
a
, E.V. Krushinov
a
,
A.A. Sulatsky
a
, S.A. Vitol
a
, V.V. Gusarov
b
, F. Fichot
c
, B. Michel
c
, P. Piluso
d
, R. Le Tellier
d
,
M. Fischer
e
, C. Le Guennic
f
, N. Bakouta
f
a
Alexandrov Research Institute of Technology (NITI), Sosnovy Bor, LR, Russia
b
Ioffe Institute, St. Petersburg, Russia
c
Institut de Radioprotection et de Sûreté Nucléaire (IRSN), St Paul lez Durance, France
d
CEA Cadarache-DEN/DTN/STRI, France
e
AREVA NP GmbH, Erlangen, Germany
f
EDF, Saclay, France
ABSTRACT
Non-steady physicochemical phenomena in the three-liquid molten pool of prototypic corium are studied in the
context of in-vessel melt retention problem. Experiments are made on the Rasplav-3 test facility within the
CORDEB program. Structure of the initial molten pool consists of the surface light melt of molten steel, the
intermediate layer of oxidic melt separated from steel melt by the crust; and the bottom layer of heavy metallic
melt. It is determined that the three-layer pool structure can stay stable for a certain period of time, but the
partitioning of steel and oxidic melt components through the crust brings the possibility of transformation of the
three-layer pool to a two-layer structure.
1. Introduction
One of the phenomena limiting the in-vessel melt retention (IVR)
during a severe accident with core meltdown in a Light Water Reactor
(LWR) is the focusing effect along the top metallic layer of the oxidic-
metallic pool, which determines the maximum heat flux applied to the
vessel wall. Comparison of this flux with DNB (departure from nucleate
boiling) on the outside of the water-cooled reactor vessel surface gives
the safety margin. The most systematic study of this problem was made
in (Theofanous et al., 1997). In a general case the intensity of focusing
effect increases, when the depth of top metal layer or stainless steel (SS)
mass decreases.
An additional complexity in the problem solution was brought by
the results of studies carried out within the OECD MASCA program. In
(Asmolov et al., 2004, 2007), in particular, it was established that
component partitioning in the system of the melted suboxidized
UO
2
+ ZrO
2
+ Zr corium and SS in the miscibility gap produces a two-
layer oxidic-metallic pool, and its metallic liquid, beside SS compo-
nents, includes U, Zr and a small amount of O. Depending on the system
composition, the metallic liquid density can be either lower or higher
than the oxidic liquid density. Therefore, the oxidic and metallic liquids
can take both bottom and top position in the molten pool. Other con-
ditions being equal, the lower SS fraction in the system is, the larger is U
fraction in the metallic liquid, and the higher is its density. Experi-
mental data on the metallic liquid composition provided in (Asmolov
et al., 2004, 2007) are close to the data of (Barrachin and Defoort,
2004; Salay and Fichot, 2004) calculated using the NUCLEA thermo-
chemical database and minimization of the Gibbs energy. The MASCA
data are used for the modelling of molten pool structure and assessment
of risks related to the focusing effect produced by the top metallic layer
(Zhang et al., 2010; Le Tellier et al., 2015).
In principle, a multi-component system can have thermo-
dynamically stable coexistence of two, three and more liquid phases. A
most frequent case is the coexistence of metallic liquid with two oxidic
liquid phases. Such stratification, for example, can be caused by the
interaction of corium with certain oxidic materials (Gusarov et al.,
2007; Asmolov et al., 2007). There are also publications on the strati-
fication of metallic melt into three liquid phases (Konovalov et al.,
2012).
The non-equilibrium melt having two, three and more liquid phases
is also possible in presence of thermal gradient maintained in the
system (Gusarov et al., 2006), or because of the spatial separation of
https://doi.org/10.1016/j.nucengdes.2018.03.004
Received 26 October 2017; Received in revised form 1 March 2018; Accepted 3 March 2018
⁎
Corresponding author.
E-mail address: vac@mail.ru (V.I. Almjashev).
Nuclear Engineering and Design 332 (2018) 31–37
Available online 19 March 2018
0029-5493/ © 2018 Elsevier B.V. All rights reserved.
T