ISSN 0021-3640, JETP Letters, 2012, Vol. 96, No. 12, pp. 759–764. © Pleiades Publishing, Inc., 2012.
Original Russian Text © N.S. Lapshina, R.E. Noskov, Yu.S. Kivshar, 2012, published in Pis’ma v Zhurnal Eksperimental’noi i Teoreticheskoi Fiziki, 2012, Vol. 96, No. 12, pp. 849–
854.
759
1. INTRODUCTION
In the current usage, nanoantennas refer to devices
for converting the angular and frequency characteris-
tics of optical radiation at subwavelength scales. Stud-
ies on nanoantennas represent a rapidly progressing
area of modern optics in view of a large number of
potential applications, which include thin-film solar
cells, chemical and biological sensors, and ultrafast
optical information processing devices [1–3]. A factor
important for most of these applications is the possi-
bility of active control over the radiation (scattering)
pattern of a nanoantenna. However, the operating
principle of most nanoantennas relies on the use of a
single mode, the one enabling the best directivity and
(or) Purcell factor [4, 5]. Nevertheless, methods have
recently been proposed for steering the radiation
(scattering) pattern via switching between different
modal regimes upon the variation of the frequency in
nanoantennas with broken geometrical or material
symmetry [6, 7] or variation of the field intensity in
nanoantennas with nonlinear components [8–14].
Here, we suggest a new concept of active dynamic
control over the scattering pattern of the nanoantenna
by using modulational instability. We demonstrate that
the onset of this instability in a nanodimer consisting
of two spherical silver nanoparticles may result in
dynamic energy exchange between the eigenmodes of
the system, which is accompanied by periodic rotation
of the scattering pattern similar to that in classical
phased-array antennas [15].
2. THEORETICAL MODEL OF A NONLINEAR
PLASMONIC NANOANTENNA
We consider a nanoantenna consisting of two iden-
tical spherical nanoparticles placed close to each other
in a silica host with the relative permittivity ε
h
= 2.15.
Let the particle radius a and the spacing d between the
centers of the spheres be 10 and 30 nm, respectively.
Under the condition a/d ≤ 1/3, the response of the
particles can be described in the dipole approximation
[16]. Assuming the nanoparticles made of silver with a
Kerr-type nonlinear response, we take the dielectric
constant in the form = + χ
(3)
. Here, the
linear term is described by the Drude formula =
ε
∞
– /[ω(ω – iν)] with ε
∞
= 4.96, ω
p
= 9.54 eV,
and ν = 0.055 eV [17]; χ
(3)
is the cubic susceptibility;
and are the local fields within the particles.
Generally, the cubic optical susceptibility of metal-
lic nanoparticles depends on the type of metal, particle
size, frequency and duration of the incident laser radi-
ation, and some other factors [18]. In particular, the
analytical quantum model developed in [19, 20] and
later confirmed by numerical simulations [21] indi-
cates that, for 10-nm-radius silver particles driven at a
frequency close to the frequency of the surface plas-
mon resonance, the cubic susceptibility is purely real
and equals χ
(3)
3 × 10
–9
esu. This value is much larger
than the cubic susceptibility of silica (~10
15
esu [22]),
and the latter is disregarded in the following.
In this paper, we analyze the dynamic mutation of
the scattering pattern of such a nonlinear dimer
nanoantenna when the response of this structure
exhibits modulation instability.
3. BASIC EQUATIONS
We study a nanoparticle dimer driven by a plane
wave with the frequency close to the frequency of the
surface plasmon resonance of an individual particle at
ε
Ag
NL
ε
Ag
L
E
12 ,
in ( )
2
ε
Ag
L
ω
p
2
E
12 ,
in ( )
Nonlinear Nanoantenna with Self-Tunable Scattering Pattern
N. S. Lapshina
a
, R. E. Noskov
a
, and Yu. S. Kivshar
a, b
a
National Research University of Information Technologies, Mechanics, and Optics, St. Petersburg, 197101 Russia
e-mail: n.lapshina@phoi.ifmo.ru
b
Nonlinear Physics Centre, Research School of Physics and Engineering, Australian National University, Canberra, Australia
Received October 9, 2012
A new concept of a nonlinear plasmonic nanoantenna with self-tunable scattering pattern (indicatrix) is sug-
gested. It is shown that the onset of modulational instability in a nanoantenna consisting of two identical non-
linear metallic nanoparticles results in dynamic energy exchange between the eigenmodes of the nanodimer,
accompanied by periodic rotation and switching of the scattering pattern. Such a nanoantenna features a
wide scanning sector, a relatively low working threshold, and a short response time. This makes it attractive
for applications in nanophotonics and biology.
DOI: 10.1134/S0021364012240071