Preparation of SiO
2
-Na
2
O-CaO-P
2
O
5
Glass-Ceramic from Waste Materials
and Heat Treatment Effects on its Morphology
N.F. Baharuddin Pallan
1,a*
, K.A. Matori
1,b
, M. Hashim
1,c
, W.F. Lim
1,d
,
H.J. Quah
1,e
, A.N. Fauzana
1,f
, N. Rosnah
1,g
, M.Z.A. Khiri
1,h
, S. Farhana
1,i
,
Z. Norhazlin
2,j
, N.A. Zarifah
3,k
, M. Nurzilla
3,l
, M.Z.M. Hafiz
3m
, C.W. Loy
3,n
,
M.I.M. Zamratul
3,o
1
Institute of Advanced Technology, Universiti Putra Malaysia,
43400 Serdang, Selangor Malaysia
2
Department of Chemistry, Faculty of Science, Universiti Putra Malaysia,
43400 Serdang, Selangor Malaysia
3
Department of Physics, Faculty of Science, Universiti Putra Malaysia,
43400 Serdang, Selangor Malaysia
a
nurfadilahbaharuddin@gmail.com,
b
khamirul@upm.edu.my,
c
mansor@upm.edu.my,
d
wayfoong317@yahoo.com.sg,
e
jinquah1st@hotmail.com,
f
fauzana22@yahoo.com,
g
rnawang@upm.edu.my,
h
mzulhasif@gmail.com,
i
nfarhanasamsudin@gmail.com,
j
norhazlin@upm.edu.my,
k
zarifah_alassan@yahoo,
l
nurzilla@gmail.com,
m
mhmzaid@gmail.com,
n
aaron_loy_41f@hotmail.com,
o
zamrah48@gmail.com
Keywords: Glass-ceramic, Solid State, Soda Lime Silica, Clam Shell, Waste Materials
Abstract. Currently, many researchers interested studying waste materials to recycle them or reuse
them in new products. From the sustainable perspective development, it is necessary to implement
new technologies to help reduce waste and thus minimize the environmental problems associated
with disposal. In this study, the preparation of SiO
2
-Na
2
O-CaO-P
2
O
5
(SNCP) glass-ceramic is
composed of Soda Lime Silicate (SLS), Clam Shell (CS), Na
2
CO
3
and P
2
O
5
in the ratio of 50: 25:
20: 5 respectively. The waste materials that were used for fabricate glass-ceramic are SLS and CS.
All the compounds were mixed to fabricate the SNCP glass-ceramic through solid state reaction.
The samples were investigated through X-ray diffraction (XRD), field emission microscope
(FESEM) and density measurement. The samples were sintered at temperature 550°C, 650°C,
750°C, 850°C until 950°C. The main phase obtained from XRD analysis is Sodium Calcium
Silicate, Na
2
CaSiO
4
with cubic crystal system at 550°C. The highest intensity phase of the
diffraction peak is (220) and at the angle 33.7°. There was new peak presence at right side of the
main phase Na
2
CaSiO
4
, which belong to Silicon Phosphate, SiP
2
O
7
at 650°C and 750°C. When heat
treatment increased at 850°C - 950°C, the main phase is Combeite, Na
4
Ca
4
(Si
6
O
18
) at diffraction
peak (220) with rhombohedral crystal system which is assigned to high crystallization temperature
(T
c
). The density of samples increases at 550°C - 750°C and decreases when heat treatment 850°C -
950°C. Sample density decreases at heat treatment 850°C - 950°C due to increases of sample lattice
parameter. FESEM analysis showed that the grain size and porosity increased when the heat
treatment increased.
INTRODUCTION
A lot of research has been carried out to find out the substitute to support the bone in the medical
field. Ceramic composites enjoy superiority due to similarity with bone minerals, exhibiting
biocompatibility and are able to be shaped into definite size. Composite ceramic play a key role for
the choice of bioceramic according to the site of implantation and their broad implication as
implants. Nowadays, bioceramics are the better alternatives since they have high corrosion
resistance, better compressive strength and relatively low density and low weight [1]. SNCP glass-
Materials Science Forum Submitted: 2015-01-11
ISSN: 1662-9752, Vol. 846, pp 189-192 Revised: 2015-09-27
doi:10.4028/www.scientific.net/MSF.846.189 Accepted: 2015-09-30
© 2016 Trans Tech Publications, Switzerland Online: 2016-03-04
All rights reserved. No part of contents of this paper may be reproduced or transmitted in any form or by any means without the written permission of Trans
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