Desalination 229 (2008) 279–293
*Corresponding author.
Some thiazole derivatives as corrosion inhibitors for carbon
steel in acidic medium
A.A. Al-Sarawy
a
, A.S. Fouda
b
, W.A. Shehab El-Dein
a*
a
Department of Mathematics and Physical Science, Faculty of Engineering, Mansoura University, Mansoura, Egypt
Tel. +20 123252770; Fax +20 502224469; email: waleedazmy1967@yahoo.com
b
Department of Chemistry, Faculty of Science, Mansoura University, Mansoura, Egypt
Received 7 February 2006; accepted revised 20 September 2007
Abstract
The effect of some prepared compounds, namely thiazole derivatives on the corrosion of C-steel in 2 M HCl
solutions has been studied using the weight loss and electrochemical polarization methods. The results showed that
the inhibition efficiency of the investigated compounds was found to depend on the concentration and the nature of
the inhibitor. The presence of the substituted donating group (–OCH
3
) plays an important role in the inhibition
percentage of these investigated compounds. The effect of temperature on the corrosion behavior of C-steel in 2 M
HCl without and with the inhibitors was studied in the temperature range from 30 to 50°C. The activation and
thermodynamic parameters E
*
a,
ΔH
*
and ΔS
*
were calculated. The inhibitors were adsorbed on the C-steel surface
according to Frumkin’s adsorption isotherm. The synergistic effect of some cations (Cu
2+
, Ni
2+
, Co
2+
and Ca
2+
) on
the corrosion inhibition of C-steel in 2 M HCl in the presence and absence of the investigated compounds was also
studied by the weight loss method.
Keywords: Corrosion inhibitor; Thiazole derivatives; C-steel; Weight loss method; Galvanostatic polarization method;
Frumkin’s isotherm
1. Introduction
The industrial consumption and development
of new corrosion inhibitors have continuously in-
creased because this corrosion control technique
is one of the most effective and economical meth-
ods to protect metal corrosion in acidic medium
[1,2]. The development of corrosion inhibitors is
based on organic compounds containing nitrogen,
oxygen, sulfur atoms, and multiple bonds in the
molecules that facilitate adsorption on the metal
surface [3]. The corrosion inhibition efficiency of
organic compounds is related to their adsorption
properties. Adsorption depends on the nature and
the state of the metal surface, on the type of cor-
rosive medium and on the chemical structure of
doi:10.1016/j.desal.2007.09.013
0011-9164/08/$– See front matter © 2008 Published by Elsevier B.V.