Materials Science and Engineering, A178 (1994) 19-22 19
Structure of diatomic clusters
Marco Ronchetti and Stefano Cozzini
Dipartimento di Fisica, Universitd di Trento, 38050 Povo (TN) (Italy)
Abstract
We investigate the structure of 13-particle clusters in binary alloys for various size ratios and concentrations to predict
which systemsare likely to form local icosahedral structures when rapidly supercooledfrom the melt.
1. Introduction
Metallic glasses would not exist in a two-dimen-
sional world. In fact, by minimizing the volume of small
clusters of equal disks one gets hexagonal structures.
Two-dimensional crystals also exhibit extended hexag-
onal order; therefore a natural, easy path exists and
leads from small structures to extended ones. The
picture is quite different in the three-dimensional
world: small clusters of equal balls are dominated by
icosahedral ordering, but the closest packing of
extended structures exhibits cubic symmetry (FCC).
Growing from small structures which optimize space
filling on a small scale to structures which do so on a
large scale requires large rearrangements. These geo-
metric considerations are true also from an energetic
point of view: the energy of a 13-atom icosahedral
cluster is significantly lower than the energy of corre-
spondent FCC or HCP clusters; for a Lennard-Jones
potential (LJ) the difference is as much as 8%, and a
similar preference for local icosahedral order is shown
by purely repulsive r -n potentials. The competition
between the preferred local structure and the optimal
extended one gives rise to frustration, as discussed in
depth by Nelson and Spaepen [1].
Steinhardt et al. [2, 3] suggested the importance of
(extended) icosahedral order in monoatomic LJ super-
cooled liquids. Honeycutt and Andersen [4] showed
that the lowest energy structures in LJ clusters are ico-
sahedral up to a size of 5000 atoms. Nos~ and
Yonezawa [5] reported that there is an increase in local
icosahedral structure during the quenching process on
LJ liquids. Similar results were obtained by Tanaka [6]
on a rubidium system and by Tsumuraya and Watanabe
[7] on a metallic system (Na) with a potential which
shows Friedel oscillations. Recently, Dzugutov [8]
reported enhanced icosahedral local order in mono-
atomic samples by using a potential which resembles
an effective metallic potential and makes the formation
of FCC more difficult. Rather surprisingly, such a
potential leads the same system to form a dodecagonal
quasicrystal [9].
On the other hand, for glasses of a binary system the
scenario is not unique. Nelson and Spaepen [1] suggest
that a small concentration of large particles should
favour the onset icosahedral order. Jonsson and
Andersen [10] reported a large amount of icosahedrai
clusters in their simulations, while Dasgupta et al. [11 ]
and Ernst et al. [12] did not find such structures.
In the present work we study the structure of
13-atom binary clusters in order to contribute to the
understanding of these contrasting results. Our objec-
tive is twofold: we wish to derive a detailed map of the
potential energy minima with respect to the concentra-
tion of small atoms in the clusters, and we intend to
explore these minimal energy configurations from a
structural point of view.
2. Simulation method
Our simulation method was the molecular dynamics
technique (see ref. 13 for an introduction to this
method). We used an LJ potential with parameters for
the large atoms (oll and e11) suited for argon. The
potential for the second atomic specie was defined by
parameters and ce22 = Cell and 022 = 1711 , where ct is the
radii-ratio. The interaction between unlike particles
was defined by Cel2 = Ce22 = Cell and 012=(01t + 022)/2.
The mass is not a relevant parameter when only struc-
tural properties are of interest, and we therefore used
equal masses for the two species. We studied 13-atom
clusters for three values of a (1.6, 1.4, 1.25), and for all
possible values of concentration ~//13. (The limiting
cases r/= 0 and r/= 13 are equivalent and well known,
since they correspond to a monoatomic system.)
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