ISSN 10274510, Journal of Surface Investigation. Xray, Synchrotron and Neutron Techniques, 2014, Vol. 8, No. 3, pp. 444–455. © Pleiades Publishing, Ltd., 2014.
Original Russian Text © L.I. Goray, M.N. Lubov, 2014, published in Poverkhnost’. Rentgenovskie, Sinkhrotronnye i Neitronnye Issledovaniya, 2014, No. 5, pp. 39–51.
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INTRODUCTION
Progress in the manufacture of Xray multilayer
diffraction gratings and mirrors with preselected
boundary shapes and assigned subatomic roughnesses
is related first of all to the holographic and litho
graphic methods used in the production thereof,
advances in material chemistry, the advancement of
vacuum techniques and technology for preparing and
treating Si plates, and achievements in nanometrology.
Further investigations are urgent because there is a
necessity to create uptodate highresolution and
highefficiency components for optical and electronic
devices (including those for 6.Xnm lithography) and
Xray freeelectron lasers and develop resonant inelas
tic Xray scattering, soft Xray and extreme UV (EUV)
astrophysics, Xray microscopy, and other fields of
application. The comparison of scattering intensities
measured with the help of synchrotronradiation (SR)
sources and Xray freeelectron lasers with data calcu
lated via rigorous methods becomes more and more
important for shortwavelength optics.
It should be emphasized that microscopy methods,
such as transmission electron microscopy (TEM),
atomicforce microscopy (AFM), and nearfield
scanning optical microscopy, are finding wide applica
tion in qualitative research into the evolution of thin
film boundary profiles. The first approach is expensive
and destructive, and the other two techniques make it
impossible to determine the boundary profiles of the
internal layers of prepared samples. Moreover, only
the local characteristics of a formed structure can be
studied with the use of microscopy methods.
The most universal approach to examination of the
morphology and composition of layers is the reflecto
metry (scatterometry) method, including its short
wavelength variant whereby the nanorelief character
istics of practically all thinfilm materials can accu
rately be determined in an integrated way [1]. When
solving the imperfectly and ambiguously defined
inverse problems of reflectometry [2], it is especially
important to have a universal and rigorous method for
solving a direct problem and information on the
recovered relief and/or refractive indices of the mate
rials, which are employed as an initial approxima
tion.Despite the substantial progress in the develop
ment of accurate numerical methods for examining
wave diffraction by arbitrary boundary asperities
achieved in the last few years [3], the Xray and neu
tron scattering intensities have only recently been ana
lyzed by means of asymptotic and approximate
approaches: the Kirchhoff scalar integral method, the
Born approximation, the distortedwave Born approx
Nonlinear Continual Growth Model of Nonuniformly Scaled Reliefs
as Applied to the Rigorous Analysis of the Xray Scattering Intensity
of Multilayer Mirrors and Gratings
L. I. Goray
a, b
and M. N. Lubov
a, c
a
St. Petersburg Academic University–Nanotechnology Research and Education Centre, Russian Academy of Sciences,
St. Petersburg, Russia
b
Institute for Analytical Instrumentation, Russian Academy of Sciences, St. Petersburg, Russia
c
Ioffe Physical Technical Institute, Russian Academy of Sciences, St. Petersburg, Russia
Received May 30, 2013
Abstract—It is revealed that certain terms entering into the nonlinear continual equation describing thin
film growth enable its application to the simulation of the surfaces of multilayer mirrors and gratings with a
large height and/or jumps of boundaryprofile gradients. The proposed model characterizes both variations
in the power spectraldensity function of the surface of Al/Zr multilayer mirrors and the smoothing and shift
of the boundaries of Mo/Si and Al/Zr gratings grown on Si substrates with triangular groove profiles by means
of magnetron and ionbeam deposition. Rigorous calculations indicate that the intensities of diffuse Xray
scattering by Au mirrors, which have similar boundary profiles with Gaussian and exponential autocorrela
tion functions, differ substantially from each other. Computer simulation of the growth of Mo/Si and Al/Zr
multilayer gratings is performed. On the basis of the calculated boundary profiles, the absolute diffraction
efficiencies of the Mo/Si and Al/Zr gratings are found via the integral equation method in the extreme UV
region. It is demonstrated that the proposed comprehensive approach to calculations of the boundary profiles
and the intensities of shortwavelength scattering from multilayer mirrors and gratings makes it possible to
carry out studies comparable in accuracy to measurements based on synchrotron radiation.
DOI: 10.1134/S1027451014030057