INSTITUTE OF PHYSICS PUBLISHING JOURNAL OF PHYSICS B: ATOMIC, MOLECULAR AND OPTICAL PHYSICS
J. Phys. B: At. Mol. Opt. Phys. 34 (2001) 1–13 PII: S0953-4075(01)21572-7
Positronium formation in positron–simple metal
clusters collisions
B/121572/P PROC
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Printed: 28/9/2001
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O A Foj ´ on
1
, R D Rivarola
1
, J Hanssen
2
and P A Hervieux
2
1
Instituto de F´ ısica Rosario, CONICET-UNR and Escuela de Ciencias Exactas y Naturales,
Facultad de Ciencias Exactas, Ingenier´ ıa y Agrimensura, Av. Pellegrini 250, 2000 Rosario,
Argentina
2
Laboratoire de Physique Mol´ eculaire et des Collisions, Institut de Physique Rue Arago,
Technopˆ ole 2000, 57078 Metz Cedex 3, France
Received 31 January 2001, in final form 24 July 2001
Published
Online at stacks.iop.org/JPhysB/34
Abstract
Positronium formation through electron capture from ground-state closed-shell
sodium clusters is studied theoretically at intermediate impact energies. The
charge transfer process is described in the independent electron model by a
continuum distorted-wave approximation. In this approximation, distortions in
the final state are introduced by using two Coulomb wavefunctions associated
with the positron- and electron-residual target interactions. The cluster is
described within the framework of the spherical background jellium model and
the Kohn–Sham formalism with a local-density approximation that includes
exchange, correlation, and a self-interaction correction. Using a partial-wave
technique, differential and total cross sections for the isoelectronic neutral and
charged closed-shell sodium clusters Na
20
, Na
-
19
and Na
+
21
are computed and
compared with the predictions of the Coulomb–Born type approximation which
neglects the distortions in the final state.
1. Introduction
Collisions of positrons impacting on atoms (ions) have been the subject of active research
over the last few years, partly motivated by the measurements obtained with the presently
available high-intensity positron beams. There are interesting reviews on the issue (see, for
instance, [1, 2]).
A continuum distorted-wave final-state (CDW-FS) approximation has been developed
to study positron–hydrogenic atom (ion) [3–5] and positron–alkali atom collisions [6]. A
four-body CDW-FS (CDW-FS-4b) model has been developed recently to study the collision
positron–alkali-earth metal [7] and positron–metastable helium [8]. In CDW-FS, the final state
of the collision is distorted by two Coulomb wavefunctions associated with the positron- and
electron residual target interactions. In this way, higher-order terms are included to describe
the collision process.
0953-4075/01/000001+13$30.00 © 2001 IOP Publishing Ltd Printed in the UK 1