S1
Supporting Information for
Pyrroloquinoline quinone maintains redox activity when bound to a
DNA aptamer
Ismaila Emahi, Isabel M. Mulvihill, and Dana A. Baum*
Department of Chemistry, Saint Louis University,
St. Louis, Missouri 63103, USA
* To whom correspondence should be addressed. D.A.B. – Tel: +1 314 977 2842; Fax: +1 314
977 2521; Email: dbaum1@slu.edu.
Supplemental Materials and Methods
Reagents and materials. DNA oligonucleotides were purchased from Integrated DNA
Technologies (IDT, Coralville, IA) and purified by denaturing polyacrylamide gel
electrophoresis (PAGE) using 1X TBE running buffer (89 mM each of Tris and boric acid, 2
mM EDTA, pH 8.3). Samples were extracted from the gel by the crush-and-soak method in TEN
buffer (10 mM Tris, pH 8.0, 1 mM EDTA, 300 mM NaCl), recovered by ethanol precipitation,
and quantified by UV absorbance.
1
The single-stranded DNA (ssDNA) random pool for in vitro
selection was 5’-GAACTAGATCGCAGC-N
70
-GGATCGAGGTAATCC-3’. The N
70
designation indicates 70 nucleotides with equimolar incorporation of the four DNA bases A, C,
G and T at each position. Two primers, primer 1: 5’-CAACAACAACAA-X-
GGATTACCTCGATCC-3’ and primer 2: 5’–GAACTAGATCGCAGC-3’, anneal to the 3’ and
5’-ends of the random pool, respectively, during PCR amplification. The non-amplifiable spacer
18 linker in primer 1 (designated as X) allows for separation of the inactive complement from the
active pool sequence via PAGE following PCR. The sequence of the unstructured DNA oligo
used in the control experiments was 5’-GAACTAGATCGCAGC-(CAA)
23
-
CGGATCGAGGTAATCC-3’. PQQ was purchased from Berry & Associates, Inc (Dexter, MI).
2,6-dichlorophenolindophenol (DCPIP) was purchased from Fisher Science Education
(Nazareth, PA). Sodium ascorbate was obtained from Sigma-Aldrich Co. (St. Louis, MO).
In vitro selection. DNA aptamers for PQQ were identified through in vitro selection (Figure S1)
using the random pool described above. PQQ was coupled to MagnaBind amine-derivatized
beads (Thermo Fisher) using 50 mM 4-(4, 6-Dimethoxy-1, 3, 5-triazin-2-yl)-4-
methylmorpholinium (DMT-MM) in 100 mM MOPS pH 7.0 and 1 M NaCl. The amount of PQQ
coupled to the beads was determined spectroscopically by measuring the A
330
of the coupling
solution before and after the coupling reaction. Prior to each incubation with beads, the DNA
pool was annealed by heating to 95 °C for 3 minutes, followed by incubation on ice for 5 min in
1X HEPES annealing buffer (5 mM HEPES pH 7.5, 10 mM NaCl, and 0.1 mM EDTA).
Selections were initiated by first incubating 200 pmol of the random pool with amine-derivatized
beads that had not been coupled to PQQ. This pre-selection column was intended to remove
sequences that bind to the beads or the tether. The unbound sequences in the supernatant were
Electronic Supplementary Material (ESI) for RSC Advances.
This journal is © The Royal Society of Chemistry 2014