ResearchArticle
Functionalized-AgNPs for Long-Term Stability and Its
Applicability in the Detection of Manganese Ions
Van-Tuan Hoang ,
1,2,3
Mai Mai,
1
LeThiTam,
1
NgocPhanVu,
2,3
Nguyen Tien Khi,
2,3
Phuong Dinh Tam ,
4
Tran Quang Huy,
2,5
Anh-Tuan Le ,
2,4
Ngo Xuan Dinh,
6
and Vinh-Hoang Tran
7
1
Advanced Institute for Science and Technology (AIST), Hanoi University of Science and Technology (HUST),
1
st
Dai Co Viet Road, Hanoi, Vietnam
2
Phenikaa University Nano Institute (PHENA), Phenikaa University, Hanoi 12116, Vietnam
3
Faculty of Biotechnology, Chemistry and Environmental Engineering, Phenikaa University, Hanoi 12116, Vietnam
4
Faculty of Materials Science and Engineering, Phenikaa University, Hanoi 12116, Vietnam
5
Faculty of Electric and Electronics, Phenikaa University, Hanoi 12116, Vietnam
6
University of Transport Technology, anh Xuan District, Hanoi 12116, Vietnam
7
SchoolofChemicalEngineering,HanoiUniversityofScienceandTechnology(HUST),1
st
DaiCoVietRoad,Hanoi,Vietnam
Correspondence should be addressed to Van-Tuan Hoang; tuan.hoangvan@phenikaa-uni.edu.vn and Anh-Tuan Le; tuan.leanh@
phenikaa-uni.edu.vn
Received 6 August 2019; Revised 2 December 2019; Accepted 3 January 2020; Published 7 February 2020
Academic Editor: Gyorgy Szekely
Copyright©2020Van-TuanHoangetal.isisanopenaccessarticledistributedundertheCreativeCommonsAttributionLicense,
which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited.
In this study, silver nanoparticles (AgNPs) were functionalized by various molecules, including sodium borohydride (NaBH
4
),
polyhexamethylene biguanide hydrochloride (PHMB), and Tween 80 to investigate the long-term stabilization of AgNPs in an
aqueous dispersion. PHMB-functionalized silver nanoparticles (AgNPs/PHMB) exhibited better stability than others and could be
stored at ambient temperature for at least 180 days. In addition to creating stabilization based on the electrostatic repulsion, the
use of PHMB helped to increase the degree of stability of the colloidal AgNPs for a long time owing to strong interactions between
Ag atoms on AgNPs with nitrogen (N) positions in PHMB molecules. e formed bond led to improving maintenance ability of
the electrostatic repulsion layer among independent nanoparticles. e applicability of the as-prepared AgNPs/PHMB was also
examined for Mn
2+
detection via a colorimetric approach. e calibration curve was found to be linear over the range of
0–100 mM with a correlation coefficient of 0.97. e amine groups of PHMB brought out a cooperative effect to form of ion-
templated chelation with Mn
2+
, which caused the aggregation of AgNPs/PHMB. is suggested that the AgNPs/PHMB could be
used as a potential probe in the detection of Mn
2+
ions. More importantly, the long-term stability of AgNPs/PHMB paved a great
promising path to provide many further solutions for the producer in practical applications.
1.Introduction
Silver nanoparticles (AgNPs) possess many unique chemical
and physical properties; therefore, AgNPs have been widely
studied and exploited in various applications, including
medical, home appliances, electronics, textiles, and cosmetics
[1]. e demand for AgNPs in the world is projected to
increase, with production estimated at around 320 tons per
year [1,2]. However, the properties of AgNPs strongly depend
on their size, shape, and crystallinity. Moreover, large specific
surface area and high surface energy lead to the self-aggre-
gation of AgNPs during storing time, which considerably
decreases their activity as well as applicability. ese indicate
that the stabilization of colloidal AgNPs is one of the most
essential factors for developing practical applications [3–5].
Furthermore, the use of suitable stabilizers not only helps
prevent the aggregation of AgNPs but also increases their
activity. erefore, many recent efforts have been performed
to functionalize AgNPs by different stabilizers such as
polymer or functional molecules, which contain amine
Hindawi
Advances in Polymer Technology
Volume 2020, Article ID 9437108, 9 pages
https://doi.org/10.1155/2020/9437108