American Journal of Analytical Chemistry, 2020, 11, 129-136
https://www.scirp.org/journal/ajac
ISSN Online: 2156-8278
ISSN Print: 2156-8251
DOI: 10.4236/ajac.2020.113010 Mar. 3, 2020 129 American Journal of Analytical Chemistry
Study of the Dispersive Component of the
Surface Energy of Polylactides by Inverse Gas
Chromatography at Infinite Dilution
Carla Zarazir
1,2
, Mohamad Rajab
1,2
, Houssam Obeid
1,2
, Joumana Toufaily
1,2
, Imad Toufeili
3
,
Tayssir Hamieh
1,2*
1
Laboratory of Materials, Catalysis, Environment and Analytical Methods Laboratory (MCEMA), Lebanese University, Hadath,
Lebanon
2
Laboratory of Applied Studies to the Sustainable Development and Renewable Energies (LEADDER), EDST, Lebanese
University, Hadath, Lebanon
3
Department of Nutrition and Food Sciences, American University of Beirut (AUB), Beirut, Lebanon
Abstract
Inverse gas chromatography at infinite dilution is a powerful technique that
can be advantageously used to characterize the surface physicochemical
properties of solid substrates as oxides and polymers in both forms of powder
or fibres. In the case of polymer, this technique can be used to determine the
second order transition phenomena temperatures. This paper was devoted to
the determination of the glass transition temperature of polylactide polymer.
The dispersive component of the surface energy
d
S
γ of polylactides was de-
termined by inverse gas chromatography at infinite dilution. Various theo-
retical models were used to deduce the dispersive component of the surface
energy of the solid substrates. These models are based on the calculation of
the molecular areas of adsorbed molecules on the polymer surface: geome-
trical model, cylindrical molecular model, liquid density model, BET method,
Kiselev results and the two-dimensional Van der Waals and Redlich-Kwong
equations. The curves relative to the variation of
d
S
γ as a function of the
temperature showed a specific graph with a maximum value of
d
S
γ at a cer-
tain particular temperature characteristic to the investigated polylactide po-
lymer. In fact, the maxima of
d
S
γ indicated the presence of glass transition
temperature Tg of polylactide whatever the molecular model used. This study
showed a glass transition temperature equal to 64˚C confirming that obtained
by other studies.
Keywords
Adsorption, Surface Area, Surface Energy, Retention Volume, N-Alkanes,
How to cite this paper: Zarazir, C., Rajab,
M., Obeid, H., Toufaily, J., Toufeili, I. and
Hamieh, T. (2020) Study of the Dispersive
Component of the Surface Energy of Poly-
lactides by Inverse Gas Chromatography at
Infinite Dilution. American Journal of
Analytical Chemistry, 11, 129-136.
https://doi.org/10.4236/ajac.2020.113010
Received: January 27, 2020
Accepted: February 28, 2020
Published: March 3, 2020
Copyright © 2020 by author(s) and
Scientific Research Publishing Inc.
This work is licensed under the Creative
Commons Attribution International
License (CC BY 4.0).
http://creativecommons.org/licenses/by/4.0/
Open Access