Current Nanomaterials
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60
Current Nanomaterials 2017, 2, 60-74
REVIEW ARTICLE
Quantitative Plasmon Polarimetry and Spin Optical Effects in Plasmonics
2405-4623/17 $58.00+.00 © 2017 Bentham Science Publishers
Shubham Chandel
1,#
, Ankit K. Singh
1,#
, Angad Gupta
1
, Subir K. Ray
1
, Jalpa Soni
2
, Partha Mitra
1,
*
and Nirmalya Ghosh
1,
*
1
Department of Physical Sciences,Indian Institute of Science Education and Research (IISER) Kolkata. Mohanpur
741246, India;
2
Department of Physics, University of Gothenburg, Gothenburg 41296, Sweden
Abstract: Background:Plasmonics’ dealing with localized surface plasmon resonances in metal na-
noparticles (nanostructures) and planar metal-dielectric interfaces is a rapidly developing field and is
under recent intensive investigations owing to fundamental interests and numerous potential applica-
tions. In this regard, the polarization properties of scattered light from plasmonic systems are of para-
mount importance for gaining fundamental understanding on a number of interesting and intricate po-
larization optical effects and for their potential applications. Coupling and inter-conversion between
the spin (SAM, circular / elliptical polarization) and orbital angular momentum (OAM, phase vortex)
degrees of freedom of light leading to the so-called spin orbit interaction (SOI) of light, is one such
intriguing spin (polarization) optical effect that has recently been observed in diverse plasmonic sys-
tems. These have received particular attention because of their potential applications towards devel-
opment of novel spin-controlled nanophotonic devices.
Objective: Here, we briefly review the basic concepts of SOI, the resulting spin optical effects and
their manifestations in diverse nano-plasmonic systems.
Method: Mueller matrix spectroscopic system is developed and utilized for probing and tuning spin-
dependent plasmonics effects.
Results: We provide illustrative results on controlled enhancement of the SOI effects in plasmonic
nanostructures. The specifics of a novel dark field Mueller matrix spectroscopic experimental system
and the representative results of studies using this system on the SOI and other spin-based plasmonics
effects are presented.
Conclusion: The implications of these results towards spin-controlled photonic applications are dis-
cussed.
A R T I C L E H I S T O R Y
Received: April 05, 2017
Revised: May 29, 2017
Accepted: June 19, 2017
DOI:
10.2174/2405461502666170629141329
Keywords: Plasmonics, plamon resonance, spin orbit interaction, spin hall effect of light, polarimetry, Fano resonance.
1. INTRODUCTION
Interaction of light with noble metal nanoparticles and
nanostructures have attracted considerable current interest
due to their unique optical properties governed by the so-
called surface plasmon resonance effects [1, 2]. The surface
plasmons can either be propagating, for instance at planar
metal-dielectric interfaces, or localized as in the case of met-
al nanoparticles / nanostructures, leading to strong enhance-
ment of local electromagnetic fields. The localized plasmon
resonances, due to the inherent sensitivity of the distinctive
spectral (wavelength dependent) characteristics towards local
dielectric environment, are being pursued for numerous prac-
tical applications which include, ultra-high sensitive chemi-
cal and biomedical sensing, bio-molecular manipulation,
*Address correspondence to these authors at the Department of Physical
Sciences, Indian Institute of Science Education and Research (IISER) Kol-
kata, Nadia, India; Tel/Fax: +91 33 2587 3020;
E-mails: nghosh@iiserkol.ac.in; pmitra@iiserkol.ac.in
#
The authors contributed equally to this work.
labeling, detection, contrast enhancement in optical imaging,
surface enhanced spectroscopy (Raman and fluorescence),
development of novel nano optical devices, optical infor-
mation processing, data storage and so forth [3-9]. A number
of intriguing fundamental effects associated with the interac-
tion of light with plasmonic nanostructures have also been
observed recently. Spin orbit interaction (SOI) and Spin Hall
effect (SHE) of light [10-17], Goos–Hänchen (GH) and Im-
bert–Fedorov (IF) shifts [18, 19], helicity-independent trans-
verse spin and spin (polarization) dependent transverse mo-
mentum [12, 20], spin-momentum locking and quantum spin
hall effect [12, 21], spin controlled uni-directional excitation
of surface modes, optical analogue of quantum weak meas-
urements in plasmonic structures [22], coupled plasmons and
plasmonic Fano resonances [23, 24], are some of the intricate
plasmonic effects. Since, polarization state of light plays an
important role in the light-matter interactions leading to most
of these aforementioned effects, detailed knowledge on the
polarization transformation is crucial for fundamental under-
standing of the effects. Acquisition of complete polarization
information from plasmonic nanostructures and its analysis /