FEMS Microbiology Letters 9 (1980) 121-124
© Copyright Federation of European Microbiological Societies
Published by Elsevier/North-Holland Biomedical Press
121
EFFECT OF MOLYBDENUM STARVATION AND TUNGSTEN ON THE SYNTHESIS AND
ACTIVITY OF NITROGENASE IN ANABAENA CYLINDRICA
PATRICK C. HALLENBECK and JOHN R. BENEMANN *
Sanitary EngineeringResearch Laboratory, University of California, Berkeley, CA 94 720, U.S.A.
Received 23 June 1980
Accepted 16 July 1980
1. Introduction
As with other nitrogen-fixing organisms, molyb-
denum is required for the growth of cyanobacteria on
atmospheric nitrogen [1 ] due to the association of
this metal with one of the two nitrogenase proteins
[2]. The results of substituting vanadium or tungsten
for molybdenum in the growth media have been dif-
ferent for different organisms [3-10]. In some cases
there is an apparent molybdenum requirement for
synthesis of nitrogenase, as in Klebsiella pneumoniae
or Clostridium pasteurianum [9,10].
Replacement of molybdenum by tungsten in the
growth medium ofAnabaena cylindrica permits the
synthesis of active nitrogenase component II [11] ;
however, nitrogenase activity itself is very low [12].
In the non-heterocystous cyanobacterium, Plecto-
nema boryanum, both nitrogenase proteins appear to
be synthesized when the cultures are induced under
molybdenum-deficient conditions (with or without
tungsten) [7]. Here we have investigated the effects
of molybdenum starvation (with and without tung-
sten) on in vivo and in vitro nitrogenase activity. Our
results are consistent with the results obtained with
Plectonema boryanum; namely that the nitrogenase
proteins are synthesized in the absence of combined
nitrogen under conditions of molybdenum starvation.
* To whom inquiries should be addressed. Current address:
Ecoenergetics, Inc., 180 Viewmont Ave., Vallejo, CA 94590,
U.S.A.
2. Materials and Methods
2.1. Organism and culture methods
A. cylindrica 629 was grown in modified Allen and
Arnon media [2] made with distilled, deionized water
and with molybdenum and tungsten omitted from
the trace metal solution (nil media). These metals
were added as sodium molybdate or sodium tungstate
as needed. 2 M NH4C1 was added to a final concentra-
tion of either 5 mM NH4C1, for maintenance of stock
cultures on nil media; or 1 mM NH4C1, for growth of
cultures in which depression of heterocyst differentia-
tion was desired. (This amount of nitrogen supported
growth to about 0.245 g dry weight/.) Nitrogen-
starved cultures with active nitrogenase (grown on
media containing molybdenum) were prepared as
previously described [2]. Cultures were used when
nitrogen starvation derepression of heterocyst differ-
entiation was complete (36-48 h). The cultures were
grown as either non-axenic 47-liter or axenic 2-liter
batch cultures, and in vivo experiments were con-
ducted in either 2-liter or 250-ml culture vessels.
Lighting (2.0 • 104 erg/cm2/s), growth determina-
tions, and dry weight measurements were as previ-
ously described [13]. During nitrogen starvation and
in vivo experiments, cultures were sparged with
99.7% argon, 0.3% carbon dioxide.
In vivo [13] and in vitro [2] nitrogenase activities
were determined as previously described. Determina-
tion of component I protein was performed by a
modification of the Laurell electroimmunodiffusion
technique [14].
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