FEMS Microbiology Letters 6 (1979) 45-46
© Copyright Federation of European Microbiological Societies
Published by Elsevier/North-Holland Biomedical Press
45
ADENYLATE ENERGY CHARGE IN CHEMOORGANOTROPHIC THIOBACILLUS
FERROOXIDANS KG-4
PAIVI M. SORMUNEN * and OLLI H. TUOVINEN **
Department of General Microbiology, University of Helsinki, SF-O01 O0 Helsinki 1O, and Department of Microbiology, University
of Helsinki, SF-00710 Helsinki 71, Finland
Received 19 March 1979
1. Introduction
The adenylate energy charge is a measure of the
cellular adenine nucleotide pool indicating the ener-
getic state and the overall metabolic regulation of
energy generation and expenditure [1-3] :
ATP + 0.5 ADP
ATP + ADP + AMP
In active cells not subjected to metabolic stress or
deprivation, the energy charge has been shown to
stabilize within the range of 0.8-0.9 [ 1,4]. In the
present study the adenylate energy charge was mo-
nitored during the growth of a heterotrophic strain
of Thiobacillus ferrooxidans. The results show that
the energy charge values are comparable to those
reported for other microorganisms. Furthermore, the
energy charge is shown to indicate metabolic changes,
possibly such as diauxie, which may not be apparent
by the conventional measures of growth.
2. Materials and Methods
T. ferrooxidans strain KG-4 was originally supplied
by Dr. F. Shafia (California State Polytechnic College,
Pomona, CA 91768) and maintained on glucose [5,
6]. Growth experiments were carried out using 50 ml
* Present addresses: Lumatek Ltd., P.O. Box 9, SF-02211
Espoo 21, Finland; ** Department of Microbiology, The
Ohio State University, Columbus, Ohio 43210, U.S.A.
cultures in 250 ml shake flasks at 180 rev./min and
28°C. The growth on glucose was followed by mea-
surement of absorbance at 440 nm. 1-ml samples of
cultures were taken at intervals for determination of
adenine nucleotides. A survey of the literature
indicated that a varying proportion of the intra-cellu-
lar nucleotides may escape to the medium if the
bacteria are first filtered or centrifuged [7,8] : the
size of this fraction is greatly dependent on the
physiological condition of the bacteria. In the present
study, therefore, only the total adenine nucleotide
pool in the samples was determined. (Normally the
extracellular level of nucleotides is almost negligible
in comparison to their intracellular pool). Samples
were extracted with perchloric acid followed by
neutralization and the enzymic conversion of AMP
and ADP by the myokinase and pyruvate kinase reac-
tion as described in detail by Ball and Atkinson [9].
ATP was assayed by the luciferine-luciferase bio-
luminescence reaction using a Lumac Celltester (Lu-
mac Systems AG, Basel) to monitor the light emis-
sion. All the reagents including the stocks of AMP,
ADP and ATP were checked for purity with respect
to contaminating adenine phosphonucleotides. The
myokinase and pyruvate kinase enzymes were pur-
chased from Sigma Chemical Co. and Boehringer
GmbH, respectively, and checked for purity. The
luciferine-luciferase enzyme of Pholinus pyralis
was obtained from Lumac Systems AG (Lumit NS).
The recovery of known amounts of nucleotides using
the entire procedure of extraction, enzymic conver-
sion and measurement varied between 92-102%. The
recovery was routinely determined when measuring
different batches of samples.
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