ELSEVIER Physica B 210 (1995) 121-130
Origin of the shallow oxygen levels in perovskite structures
M.D. Glinchuk, R.O. Kuzian, A.A. Karmazin
Institute for Material Sciences, Ukrainian Academy of Sciences, Krjijanovskogo Street 3, 252180 Kiev, Ukraine
Received 5 August 1994
Abstract
A mechanism of shallow oxygen level formation in band gap of perovskites is proposed. It is shown that local lattice
distortions lead to such levels. Three types of neutral impurities as well as BO 6 cluster ionization were considered as the
reason of oxygen ion displacements. The electronic structure calculation of distorted crystal was carried out analytically
in the framework of LCAO model. It was seen that energy level values depend on geometry of distortions. Applicability of
the obtained result to the explanation of shallow O- levels observed in BaTiO3 recently is discussed.
1. Introduction
In the last years several experimental evidences
about existence of shallow impurities levels in the
band gap of the dielectric crystals with perovskite
structure appeared. Nowadays these shallow levels
are known to play an important role in photocon-
ductivity, photoluminescence and photorefractive
effects. E.g. transformation of blue photolumines-
cence line into yellow one was observed in undoped
KTaO3 at T I> 50 K so that there was only yellow
line at T/> 80 K [1]. The authors explained these
results by existence of unknown nature shallow
(~< 80 K) levels in KTaO3 band gap. Under the
light beam these levels trap holes from valence
band at low temperature and lose them at T higher
than 80 K. The explanation of observed depend-
ence of photoconductivity on light intensity in
BaTiO3 also requires that one of the centers is
connected with shallow levels [2]. On the other
hand ESR signals of O- paramagnetic centers were
identified recently in BaTiO3 and other single crys-
tals (see Ref. [3] and references therein) after low
temperature illumination. The existence of three types
of O- centers with energies about 25, 40 and 65 K,
respectively, was shown in nominally undoped
BaTiO3. The distribution of internal strains was
supposed to be the reason for O- centers variety.
In another nominally undoped BaTiO3 it was iden-
tified that holes created by low temperature illu-
mination were captured at 0 2- ions next to A13 ÷
substituted for Ti 4 +. Two shallow O- trapped hole
centers in BaTiO3 were identified [4] to arise from
association with Na ÷ and Pt x ÷. After ),-irradiation
O - paramagnetic centers were observed in congru-
ent LiNbO3 [5]. Recently observation of photo-
conductivity in undoped Kl-xLixTaO3 at low
temperature region (T < 80 K) was explained with
the help of oxygen shallow levels originating from
the shifted 0 2 - ions next to off-center Li + ions [6].
In this work we have shown that in the common
case shallow oxygen levels appear in the band gap
of the crystals of a perovskite structure with defects
due to oxygen ions displacements. Three types of
neutral impurities as well as BO 6 cluster ionization
were considered as the reason for oxygen ions dis-
placements. The calculation of electronic structure
was carried out analytically in the framework of
LCAO model allowing for interactions between
nearest and next-nearest neighbors. It was shown
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