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Molecular and Cellular Biochemistry 253: 21–29, 2003.
© 2003 Kluwer Academic Publishers. Printed in the Netherlands.
Spectroscopic, structural and antibacterial
properties of copper(II) complexes with bio-
relevant 5-methyl-3-formylpyrazole N(4)-benzyl-
N(4)-methylthiosemicarbazone
Dhiman Kumar Sau,
1
Ray J. Butcher,
2
Siddhartha Chaudhuri
3
and
Nityananda Saha
1
1
Department of Chemistry, University of Calcutta, Kolkata, India;
2
Department of Chemistry, Howard University, Washington,
DC, USA;
3
RSIC, Bose Institute, Kolkata, India
Abstract
The coordination behaviour of the title ligand, 5-methyl-3-formylpyrazole N(4)-benzyl-N(4)-methylthiosemicarbazone
(HMPz4BM), is reported with solid state isolation of copper(II) complexes, [Cu(HMPz4BM)X
2
] (X = Cl, Br, NO
3
, ClO
4
and
BF
4
) which have been spectroscopically and structurally characterised. I.r. data for the free ligand and its Cu(II) complexes
indicate that HMPz4BM exhibits a neutral NNS tridentate function via the pyrazolyl nitrogen(tertiary), azomethine nitrogen
and thione sulphur. Electronic spectral data are suggestive of a square pyramidal environment for the seemingly pentacoordinated
Cu(II) species. E.s.r parameters (RT and LNT) of the reported copper(II) complexes are indicative of a d
x2–y2
ground state for
the reported species. Cyclic voltammograms of Cu(II) complexes show a quasireversible Cu
II
/Cu
III
couple and also an irrevers-
ible Cu
II
/Cu
I
couple. X-ray crystallography of a representative species, [Cu(HMPz4BM)(NO
3
)
2
] (C2/c, monoclinic), has unam-
biguously documented the conjectural findings from i.r. data that coordinating sites of the title ligand are pyrazolyl (tertiary) nitrogen,
azomethine nitrogen and the thione sulphur (NNS); and the oxygen of one of the nitrate ions has occupied the basal plane; the
fifth coordination position has been occupied by the oxygen of another nitrate ion in a square pyramidal geometry. The antibac-
terial properties of the ligand and its copper(II) complexes studied on microorganism, Staphylococcus aureus have pointed out
that most of the complexes have higher activities than that of the free ligand. (Mol Cell Biochem 253: 21–29, 2003)
Key words: pyrazole, thiosemicarbazone, copper(II) complexes, spectroscopy, X-ray crystallography
in DNA strands [4]. Moreover, recent studies have indicated
that for these ligands the coordination by the tridentate thio-
semicarbazone (tsc) moiety involving the heterocyclic atom
as well as the substitution on the terminal N(4) atom are cru-
cial for their antifungal activity [4a]. The antimicrobial activi-
ties of the copper(II) complexes of pyridyl dithiocarbazates
have been studied by Ali et al. [4b] who have found that the
parent Schiff base ligand is inactive against various bacteria,
but its square pyramidal copper(II) complexes of the type
Cu(NNS)X
2,
are remarkably active.
Introduction
Heterocyclic thiosemicarbazones and their transition metal
complexes have received considerable attention from the co-
ordination chemists, because of their well-documented bio-
logical activities like antitumor [1, 1a], antimalarial [2] and
antiviral [3] properties. Copper(II) complexes of heterocyclic
N(4)-substituted thiosemicarbazones are known to exercise
bio-activity via a mechanism involving either inhibition of
the enzyme ribonucleotide reductase, or creation of lesions
Address for offprints: N. Saha, University of Kalyani, Kalyani 741235, India (E-mail: n.saha@cucc.ernet.in; nsaha2@yahoo.com)