Two-energy-gap preformed-pair scenario for cuprate superconductors:
Implications for angle-resolved photoemission spectroscopy
Chih-Chun Chien,
1
Yan He,
1
Qijin Chen,
2,1
and K. Levin
1
1
Department of Physics and James Franck Institute, University of Chicago, Chicago, Illinois 60637, USA
2
Department of Physics and Zhejiang Institute of Modern Physics, Zhejiang University, Hangzhou, Zhejiang 310027, China
Received 15 April 2009; published 25 June 2009
We show how, within a preformed-pair scenario for the cuprate pseudogap, the nodal and antinodal re-
sponses in angle-resolved photoemission spectroscopy necessarily have very different temperature T depen-
dences. We examine the behavior and the contrasting T dependences for a range of temperatures both below
and above T
c
. Previously, the distinct nodal and antinodal responses have provided strong support for the
“two-gap scenario” of the cuprates in which the pseudogap competes with superconductivity. Instead, our
theory supports a picture in which the pseudogap derives from pairing correlations, identifying the two-gap
components with noncondensed and condensed pairs. Our calculations are based on a microscopic diagram-
matic approach for addressing pairing correlations in a regime where the attraction is stronger than BCS and
the coherence length is anomalously short. This many body theory-based scheme takes as a starting point the
BCS ansatz for the ground-state wave function and incorporates finite temperature effects through coupled
equations for the single particle and pair propagators or T matrix. It leads to reasonably good agreement with
a range of different photoemission measurements in the moderately underdoped regime and we emphasize that
here there is no explicit curve fitting. We briefly address the more heavily underdoped regime in which the
behavior is more complex.
DOI: 10.1103/PhysRevB.79.214527 PACS numbers: 74.20.z, 74.25.Jb, 74.72.Hs, 79.60.i
I. INTRODUCTION
A. Background literature
An important dichotomy is emerging in descriptions of
the mysterious pseudogap phase of the cuprates which has
resulted in different theoretical scenarios.
1
At the heart of this
dispute is whether the pseudogap observed in the normal
state is derived from the superconductivity itself or whether
it results from a competing, but somewhat elusive order pa-
rameter. Experiments i which directly study this anomalous
normal phase have provided evidence for both points of
view.
2–5
However, there is an even larger class of recent ex-
periments ii which address the superconducting phase.
These are based on angle-resolved photoemission
6–8
and Ra-
man scattering
9,10
as well as scanning tunneling
microscopy.
11–14
They quite generally reveal that there are
two distinct temperature dependences associated with the be-
havior of the spectral function and related properties in the
nodal and antinodal regions of momentum space. The nodal
response appears to reflect superconducting order whereas
the antinodal response is much less sensitive to T
c
. For this
reason, it is speculated that the pseudogap may derive from a
competing order parameter. Finally, there is a third class of
experiments iii which probe the behavior as the system
evolves from above to just below T
c
and establish that the
transition is clearly second order. Here, for example, one sees
a very smooth evolution of the angle-resolved photoemission
spectroscopy ARPES response in the antinodal
direction.
15,16
Many other properties
17,18
which depend on
the excitation gap show no clear signature of T
c
. This is
generally interpreted as evidence in favor of a precursor-
superconductivity origin to the pseudogap.
It is the last two classes of experiments which are the
focus of this paper. Indeed, there is very little in the theoret-
ical literature which addresses these phenomena. Rather the
emphasis has been on the ground state or on the normal,
pseudogap phase. Our goal is to show how to reconcile, in
particular, the experiments of class ii with a preformed-pair
scenario. Moreover, it is possible that the arguments pre-
sented here can be viewed as “modular” in the sense of ap-
plying to alternate precursor-superconductivity approaches
such as the “phase fluctuation” approach
19
or the resonant
valence bond RVB scheme.
20
We stress that there appear to
be no counterpart studies of the intermediate temperature
broken symmetry state within the more widely espoused
phase fluctuation scheme.
19
Our explanation of the di-
chotomy is built around a picture in which the short coher-
ence length cuprates are somewhere between BCS and Bose-
Einstein condensed BEC systems. This crossover scheme
seems to be gaining in support
1,21
and is now widely studied
in the cold Fermi gases.
17,22,23
Our emphasis here is on mod-
erately underdoped cuprates where at the lowest tempera-
tures the spectral properties appear to conform to that of a
simple d-wave BCS-like state.
7,24
While the behavior ap-
pears to be much more complex in the heavily underdoped
regime, nevertheless, there is a smooth evolution with dop-
ing and all the indications for distinct nodal and antinodal
responses are present at moderate underdoping. Thus, we
feel the same qualitative physics regarding the origin of the
pseudogap is appropriate to both moderately and heavily un-
derdoped cuprates.
We build on a d-wave BCS-like ground state where the
variational parameters are determined in conjunction with a
self-consistency condition for the chemical potential, . This
self-consistent treatment of which is close to but different
from E
F
is necessary
25,26
to accommodate the relatively
short coherence length of the cuprates. Our contribution in
the past
17,27
has been to address the associated finite tempera-
PHYSICAL REVIEW B 79, 214527 2009
1098-0121/2009/7921/21452711 ©2009 The American Physical Society 214527-1