Research Article 2018, 3(4), 193-198 Advanced Materials Proceedings
Copyright © 2018 VBRI Press 193
Reduced graphene oxide-zinc oxide nano-
composites for gas sensing applications
Sitakshi Gupta, Chhaya Ravikant*
Department of Applied Sciences & Humanities, Indira Gandhi Delhi Technical University for Women, Kashmere Gate,
New Delhi-110006
*Corresponding author
DOI: 10.5185/amp.2018/025
www.vbripress.com/amp
Abstract
Nowadays, gas sensors are fast becoming an imperative part of modern life with extensive applications in domestic safety,
environmental monitoring, industrial process control, public security, medical applications and chemical warfare assessment
amongst many others. The detection of minor gas leaks has been a challenging area of research, particularly in view of the
hazards to human health and safety posed by toxic gases like NO2, NO, CO, NH3 etc and combustible gases like methane,
hydrogen gas and some volatile organic compounds. Thus it is imperative to evolve and employ simple yet reliable gas
sensing mechanisms with optimum response and selectivity towards even low concentration of analyte gas at room
temperature. Most of the conventional gas sensors are based on metal-oxide semiconductors which are low-cost, exhibit good
sensitivity and fast response/recovery. Zinc oxide is one such n-type semiconducting oxide, which has been widely studied
for gas sensing response due to its ease of fabrication, high sensitivity and environment-friendly nature. However, the
operating temperature of such sensors is usually high (>200°C) owing to the wide band-gap (3.37 eV) and high electrical
resistance (kΩ-MΩ), which limits their practical utilization. In order to be used in hazard monitoring and home/workplace
safety, the gas sensors need to be sensitive to gas exposure in mild operating conditions. As an alternative, more recently,
graphene and its derivatives like pristine graphene (PG), reduced graphene oxide (rGO) etc. have been studied for sensing
applications owing to their exceptional electronic and physical properties such as high carrier mobility at room temperature,
good thermal stability, high mechanical strength, ballistic conductivity and large specific surface area. These sensors show
high sensitivity at low operating temperatures (down to room temperature) towards low concentrations of analyte gas.
However most of these rGO based sensors exhibit relatively longer response/recovery times than metal-oxide based gas
sensors. Hence, nanocomposites formed by hybridizing graphene or its derivatives with metal-oxide nanoparticles are being
explored as gas sensing materials. Combining reduced graphene oxide with zinc oxide to form hybrid nanostructures is
particularly interesting because not only do they display the individual properties of the metal oxide NPs (faster
response/recovery times) and of graphene (high electronic conductivity leading to efficient room temperature gas response),
but may also have synergistic effects leading to better sensitivity as a gas sensing material. Here we present a review of the
recent progress in rGO-ZnO nanocomposites based gas sensors. Copyright © 2018 VBRI Press.
Keywords: Reduced graphene oxide, zinc oxide, gas sensor, grapheme.
Introduction
Gas sensors are fast becoming an imperative part of
modern life with extensive applications in domestic
safety, greenhouse gas monitoring for environmental
studies, industrial process control such as methane
detection in mines, in automotive industry for evaluating
the exhaust of cars for pollution control check, public
security, medical applications such as electronic noses
simulating human olfactory system and chemical warfare
assessment. They are being progressively employed in
mass-market applications, such as in indoor air quality
control as well as the more conventional areas of
explosive and toxic gas detection. In view of the hazards
to human health and safety posed by toxic gases like NO2,
NO, CO, NH3 etc and combustible gases like methane,
hydrogen gas, and some volatile organic compounds, it is
imperative to evolve and employ simple yet reliable gas
sensing mechanisms with optimum response and
selectivity towards even low concentration of analyte gas
at room temperature.
An efficient gas sensing technique is characterized by
certain performance parameters such as: (i) High
sensitivity (ii) Low detection limit i.e. the minimum
volume of target gas concentration at which response is
generated should be low (iii) Good selectivity which
means that the sensor should be able to detect a particular
gas from a given gas mixture (iv) Faster response time (v)
Short recovery time (vi) Operating Temperature should be
ambient (vii) Reversibility i.e. the sensing material should
return to its original state after detection is complete (viii)
Good Adsorptive capacity (ix) Low Fabrication cost (x)
Stability of Operation.