Arch Microbiol (1990) 154:192-198 Archives of
Hicrnbinlngy
© Springer-Verlag 1990
Microbial degradation of acrylamide monomer
Rishi Shanker*, Cherla Ramakrishna, and Prahlad K. Seth
Industrial Toxicology Research Centre (Gheru Campus), Post Box 80, Mahatma Gandhi Marg, Lucknow - 226001, India
Received October 17, 1989/Accepted March 8, 1990
Abstract. Acrylamide, a neurotoxic monomer with exten-
sive industrial applications was found to be degraded by
the microorganisms present in a tropical garden soil. A
bacterium capable of degrading acrylamide was isolated
from this soil by enrichment. It was found to be aerobic,
gram-negative, motile, short rod and identified as
Pseudomonas sp. The bacterium degraded high concen-
trations of acrylamide (4 g/l) to acrylic acid and ammonia
which were utilized as sole carbon and nitrogen source
for growth. An amidase was involved in the hydrolysis
of acrylamide, which could act on other short chain am-
ides like formamide and acetamide but not on acrylamide
analogues: methacrylamide and N,N-methylene bis-
acrylamide. The enzyme was sensitive to catabolite re-
pression by succinate both in presence as well as absence
of nitrogen source.
Key words: Aerobic degradation - Soil - Acrylamide -
Acrylic acid - Ammonia - Pseudomonas - Amidase
Acrylamide (ACR, CH 2 =CHCONH2) , a widely used
monomer in polymer industry is a potent neurotoxin.
Man and animals exposed to this neurotoxin show be-
havioural disorders and "dying back" type of central and
peripheral neuropathy (Tilson 1981; Shanker and Seth
1986). Acrylamide has also been observed to induce ab-
normalities in mitotic and meiotic cells in animals and
plants (Shairashi 1978; Shanker et al. 1987). Acrylamide
has a variety of industrial applications, including its use
as a grouting agent, soil stabilizer and strengthener in the
manufacture of paper and cardboards. Polyacrylamide
* Presentaddress:DepartmentofChemistry, 207ChandleeLabora-
tory, The Pennsylvania State University, University Park, PA 16802,
USA
Offprint requests to: R. Shanker
Abbreviations: Acrylamide (ACR), High Performance Liquid Chro-
matography (HPLC)
are used as flocculents in water treatment (Prasad 1982),
disposal of industrial waste and as a pusher-fluid for
increasing secondary recovery from oil wells (Tilson
1981). Unregulated commercial polyacrylamides may
contain 0.3 to 5 % monomeric acrylamide as contaminant
and industries using polyacrylamide or acrylamide-
acrylic acid copolymers discharge effluents containing
acrylamide monomer into environment (Croll et al.
1974).
The widespread application of acrylamide and its
polymers, has led to contamination of soil and water
(Cherry et al. 1956; Igisu et al. 1975). The unreacted
acrylamide from polymers has been found to migrate into
soil and subsequently into plants (Nishikawa et al. 1978,
1979) and water supplies (Igisu et al. 1975). Cases of acute
acrylamide poisoning as a result of contamination of
water supply have been reported in Japan (Igisu et al.
1975). The monomer was found to remain stable for more
than 2 months in tap water (Brown et al. 1980).
In spite of numerous reports about the microbial
degradation of acrylamide in river water (Cherry et al.
1956; Croll et al. 1974; Brown et al. 1982) and soil (Lande
et al. 1979) little is known about the nature of micro-
organisms involved in transformation of acrylamide. The
chemical nature and fate of intermediate(s) formed on
transformation of acrylamide has not been demonstrated.
In view of the toxicity of acrylamide, the present investi-
gation aimed to examine the detoxication of acrylamide
in a tropical soil as well as in bacterial culture.
Materials and methods
Chemicals
Acrylamide of analytical grade was obtained from Sigma, USA and
acrylic acid from BDH, England. All other chemicals used were of
highest purity available commercially.