S-1 Supporting Information TiO2-Coated Silica Photonic Crystal Capillaries for Plasmon- Free SERS Analysis Bing Liu, †,‡,§ Kan Wang, †,‡ Bingbing Gao, Jie Lu, Haiming Li, #, , and Xiangwei Zhao *†,‡,§ State Key Laboratory of Bioelectronics, School of Biological Science and Medical Engineering, National Demonstration Center for Experimental Biomedical Engineering Education, § Key Laboratory of Environmental Medicine Engineering of Ministry of Education, School of Materials Science and Engineering, # State Key Laboratory of Millimeter Waves, Southeast University, Nanjing 210009, China School of Pharmaceutical Sciences and School of Biotechnology and Pharmaceutical Engineering, Nanjing Tech University, Nanjing 211816, China. School of Telecommunications and Information Engineering, Nanjing University of Posts and Telecommunications, Nanjing, 210003, China Key Laboratory of Radar Imaging and Microwave Photonics, Nanjing University of Aeronautics and Astronautics, Nanjing, 210016, China *Email: xwzhao@seu.edu.cn Table of Contents Figure S1 FDTD simulation model of the TiO2-coated silica photonic crystal capillary. Figure S2 Raman and reflection spectra of the TiO2-coated silica photonic crystal capillary. Figure S3 FDTD simulation of the photonic crystal capillary. Figure S4 Reproducibility test of five batches of the TiO2-coated photonic crystal capillary. Figure S5 Raman spectra of 10 -2 M dopamine adsorbed into the bare and TiO2- coated photonic crystal capillaries. Table S1 A comparison of dopamine detection between different methods. Table S2 Detection and recovery test of dopamine in the human urine samples.