Desalination 248 (2009) 836–842
Monitoring of the quality of winery influents/effluents and
polishing of partially treated winery flows by homogeneous
Fe(II) photo-oxidation
Natasa Anastasiou
a,b
, Maria Monou
a
, Dionissios Mantzavinos
b
, Despo Kassinos
a
*
a
Department of Civil and Environmental Engineering, University of Cyprus, 75 Kallipoleos, 1678 Nicosia, Cyprus
b
Department of Environmental Engineering, Technical University of Crete, Polytechneioupolis,
GR-73100 Chania, Greece
Tel: 003522892275; Fax: 0035722892295; email: dfatta@ucy.ac.cy
Received 2 October 2008; accepted 12 November 2008
Abstract
Winery wastewaters contain high concentrations of organic compounds including phytotoxic and recalcitrant
compounds like phenols. Its treatment by conventional processes is difficult due to the variability of the character-
istics of the liquid waste. The main objectives of this work were to (1) monitor onsite the quality of winery wastes
prior to and following sequential physical and biological treatment and (2) assess the efficiency of coupling phys-
ical and biological treatment to photo-Fenton oxidation serving as the final polishing step. A partially treated
effluent with chemical oxygen demand (COD) and biochemical oxygen demand (BOD
5
) values of 1060 and
210 mg/L respectively was subject to photo-Fenton oxidation at H
2
O
2
and Fe
2+
concentrations between
34–175 and 0.5–2 mM respectively, solution pH
0
= 2.5, under continuous UV-A irradiation provided by a
125 W lamp. In general, organic matter degradation increased with increasing treatment time reaching values
of COD or BOD removal as high as 80% after 4 h of reaction. Regarding the effect of initial iron and hydrogen
peroxide concentrations, there appears to be an optimum dosage for both, above which treatment performance
deteriorated. Hence, the combined biological + photo-Fenton oxidation resulted in 95% COD removal.
Keywords: Advanced oxidation; BOD removal; COD removal; Photo-Fenton; Winery wastewaters
1. Introduction
The wine industry generates large volumes of
wastewaters originating from various washing
steps during the crushing and pressing of grapes
as well as the rinsing of fermentation tanks, bar-
rels and other items of equipment. According to
Vlyssides et al. [1], the total production of
wastewater from a winery is about 1.2 times
greater than the production of wine. Winery
wastewater is characterized by high organic con-
tent, seasonal production, unpleasant odours and
variable composition, which is associated with
the winemaking technologies employed (i.e.,
*Corresponding author.
Presented at the Conference on Protection and
Restoration of the Environment IX, Kefalonia
Greece, June 30–July 3, 2008
0011-9164/09/$– See front matter © 2009 Published by Elsevier B.V.
doi:10.1016/j.desal.2008.11.006