International Journal of the Physical Sciences Vol. 6(2), pp. 294-300, 18 January, 2011
Available online at http://www.academicjournals.org/IJPS
ISSN 1992 - 1950 ©2011 Academic Journals
Full Length Research Paper
Determination of bonding performance of several
modified wood adhesives
Mustafa Altinok
1
, Musa Atar
1
, Hakan Keskin
2
, Suleyman Korkut
3
* and Ilhan Kocaturk
1
1
Department of Furniture and Decoration, Faculty of Technical Education, Gazi University, 06500 Besevler,
Ankara, Turkey.
2
Department of Industrial Technology, Industrial Arts Education Faculty, Gazi University, 06830 Gölbasi, Ankara, Turkey.
3
Department of Forest Industrial Engineering, Faculty of Forestry, Duzce University, Beciyorukler Campus, 81620
Duzce, Turkey.
Accepted 22 December, 2010
We have assessed the effect on bonding performance of modifying synthetic wood adhesives. Wood
samples were prepared from Scots pine (Pinus sylvestris L.) and oriental beech (Fagus orientalis L.).
Samples were bonded using poly(vinyl acetate) (PVAc) and urea-formaldehyde (UF) adhesives modified
with melamine-formaldehyde (MF) and phenol-formaldehyde (PF). Modified formulations included PVAc
alone, PVAc + UF (at 15, 35 and 50% UF), UF alone, UF + MF (at 15, 35 and 50%), and UF + PF (at 15, 35
and 50% PF). Samples were exposed to three experimental environments: Standard atmosphere, cold
water, and boiling water. For bonding strength determination, we used DIN 53 255 standard. We
conclude that the adhesive modifications tested generally have no significant effect on bonding
performance under standard atmospheric conditions, but do increase bonding performance under cold
and boiling-water conditions. The best adhesive bonding strength was found using oriental beech
samples with the UF + MF (50%) adhesive: 9.24 N/mm
2
bonding strength under standard atmosphere
conditions, 6.06 N/mm
2
in cold water, and 4.39 N/mm
2
in boiling water.
Key words: Adhesive modification, poly(vinyl acetate) (PVAc), urea-formaldehyde (UF), melamine-
formaldehyde (MF), phenol-formaldehyde (PF), bonding strength, bonding performance.
INTRODUCTION
Animal-based adhesives have been widely used in
assorted industries for more than 300 years. Synthetic
adhesives provide very important technical advantages to
the woodworking industry. Synthetic adhesives are
typically either thermoplastic or duroplastic in nature.
Thermoplastic adhesives as PVAc are applied at ambient
temperature (TS EN 205). Duroplastic adhesives are
applied hot, in plasticized state, same as the
thermoplastic adhesives, but they are not cross-linked at
the time of application. Contrary to thermoplastics, these
adhesives are not plasticized again when they are
reheated. The process is not reversible.
Studies have shown that the bonding characteristics of
*Corresponding author. E-mail: suleymankorkut@hotmail.com.
synthetic adhesives can be altered when modified with
certain compounds. Plywood resistant to cold water can
be produced using Wikol (super lackleim 308) and
modified Wikol adhesives (DIN 53 255). Medium-density
fibreboard (MDF) and plywood (between 3 and 9 mm
thick), have been covered with oak, elm, teak, and
Paulownia wood panels (0.25 mm thick) using poly(vinyl
acetate) (PVAc), urea-formaldehyde (UF), and PVA/UF
adhesive mixtures. The highest bonding strengths
obtained were from PVA/UF adhesives (Gos et al., 1987).
Samples bonded with UF adhesives modified with
poly(vinyl alcohol) (1 to 2%) and amylum (10 to 15%)
were tension tested and showed increased bonding
strength (Suh et al., 1989). The UF adhesive was
modified with poly(vinyl alcohol) and amylum to increase
water resistance. The results indicated that the amount of
free formaldehyde decreased and bonding strength