Journal of Non-Crystalline Solids 147&148 (1992) 67-73
North-Holland
]OURNA L OF
NON-CffSTALLINESOLIDS
Effect of electrolyte on the gelation and aggregation of SnO 2
colloidal suspensions
Renato Satoshi Hiratsuka, Celso Valentim Santilli, Dileize Valeriano Silva
and Sandra Helena Pulcinelli
Instituto de Qufmica de Araraquara, PO Box 355, CEP 14800, Araraquara, SP, Brazil
Electrolytes may modify the physical-chemical characteristics of colloidal particle interfaces in suspension, which can
favour gel or aggregate formation. The influence of NH4CI loading on the aggregation and gelation of SnO z colloidal
suspensions was investigated using measurements of rheology, turbidity and infrared spectra. A rapid aggregate growth for
samples with CI- > 20 mM was observed. With increasing age, gelation was observed due to formation of interaggregate
bonds. For concentration of CI- between 20 and 9 raM, the aggregation process was slower allowing the formation of gel
with a network which was not destroyed as the gel was submitted to a small rate of shear. As aging continues, the
condensation reaction between OH groups gave rise to the formation of Sn-O bonds, irrespective of the electrolyte loading.
1. Introduction 2. Experimental
The preparation of SnOe-based compounds by
the sol-gel technique has received some atten-
tion in the past few years. Pathways to gel prepa-
ration from tin (II or IV) alkoxides or inorganic
salts have been investigated [1-3]. Less attention
has been paid to modeling the formation of gels
from a structural and chemical point of view,
despite their importance as precursors in the
preparation of thin layers and coatings.
Amorphous or crystalline SnOz-based materi-
als containing different degrees of hydration can
be prepared from SnC14 water solutions. Struc-
tural differences may be due to variability of
preparation conditions, of physical-chemical
characteristics of the solid-solution interface, and
of the hydrolysis and condensation reaction rate.
Otherwise, zero charge pH between 3 and 7 has
been reported [4]. The wide dispersion of data
has been attributed to sample pretreatment and
specific adsorption of cations.
In this study, conditions of hydrogel formation
from particulate tin oxide sol were investigated.
The effect of the electrolyte loading on aggrega-
tion and gelation of dispersed sols was analyzed
from rheology and spectroscopy.
Colloidal SnO 2 was prepared by precipitation
at pH 11, adding ammonium hydroxide to a SnCI 4
aqueous solution (1.0 N). The precipitate was
stored for 24 h inside the mother-liquid at 25°C.
The final electrolyte concentration (NH~-, CI-)
of suspensions was adjusted by the control of
dialysis time. Suspensions were aged in dialysis
vessels in equilibrium with the final wash water.
During aging a decrease of pH of suspensions
was observed due to the evaporation of excess
ammonia. The electrolyte loading after dialysis,
determined from the C1- concentration, and the
values of the pH measured immediately before
and after aging, are given in table 1.
The evolution of chemical and physical charac-
teristics during aging of suspensions were fol-
lowed by turbidity, Fourier transform infrared
spectra (FTIR) and steady rotational flow mea-
surements. Turbidities were determined using a
photoelectric colorimeter (Micronal-B340), mon-
ochromatic, 410 nm wavelength light. FTIR ab-
sorption spectra were measured between 100 and
4600 cm-~ using the Nicolet System with resolu-
tion less than 2 cm-~. The samples were injected
into an IR cell consisting of two KRS5 windows.
0022-3093/92/$05.00 © 1992 - Elsevier Science Publishers B.V. All rights reserved